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31. 发明授权

US06953864B2 Method for the catalytic conversion of alkylene carbonate 失效
标题翻译：碳酸亚烷基酯的催化转化方法
公开(公告)号：US06953864B2
公开(公告)日：2005-10-11
申请号：US10292172
申请日：2002-11-12
申请人： Johannes Petrus De Jonge , Jean-Paul Lange , Dennis Humphrey Louis Pello
发明人： Johannes Petrus De Jonge , Jean-Paul Lange , Dennis Humphrey Louis Pello
IPC分类号： B01J21/10 , B01J21/16 , B01J37/03 , C07B61/00 , C07C27/02 , C07C29/09 , C07C31/20 , C07C68/06 , C07C69/96
CPC分类号： C07C29/095 , B01J21/10 , B01J37/03 , C07C68/065 , Y02P20/52 , C07C69/96 , C07C31/202 , C07C31/205
摘要： A method for catalytic conversion of alkylene carbonate, wherein alkylene carbonate is contacted with C1-C5 aliphatic alcohol and/or water in the presence of Mg, Al mixed (hydr) oxide catalyst having a Mg:Al molar ratio in the range of from 4 to 20.
摘要翻译：碳酸亚烷基酯的催化转化方法，其中碳酸亚烷基酯与C 1 -C 5脂族醇和/或水在Mg，Al混合（hydr ）氧化物催化剂，其Mg:Al摩尔比在4-20范围内。

32. 发明授权

US06479557B1 Process for the preparation of hydrocarbons from carbon monoxide and hydrogen 失效
标题翻译：从一氧化碳和氢气制备烃的方法
公开(公告)号：US06479557B1
公开(公告)日：2002-11-12
申请号：US09504665
申请日：2000-02-14
申请人： Jean-Paul Lange , Ian Ernest Maxwell , Bob Scheffer
发明人： Jean-Paul Lange , Ian Ernest Maxwell , Bob Scheffer
IPC分类号： C07C2700
CPC分类号： C07C1/0485 , C07C27/06
摘要： A process for the preparation of at least two organic products from a synthesis gas by (i) converting a first synthesis gas feed to a first organic product and a first by-product; (ii) converting a second synthesis gas feed to a second organic product and a second by-product; (iii) separating the first and/or second by-product from, respectively, the first and/or second organic product, and (iv) mixing the separated first and/or second by-product with, respectively, the second and/or first organic product. Preferably, the first organic product is paraffinic hydrocarbons or oxygenates and the second organic product is olefinic hydrocarbons or oxygenates.
摘要翻译：（i）将第一合成气进料转化为第一有机产物和第一副产物从合成气中制备至少两种有机产物的方法;（ii）将第二合成气进料转化为第二有机物产品和第二副产物;（iii）将第一和/或第二副产物分别与第一和/或第二有机产物分离，和（iv）将分离的第一和/或第二副产物与第一有机产物是链烷烃或含氧化合物，第二有机产物是烯属烃或含氧化合物。

33. 发明授权

US06211406B1 Process for the manufacture of &agr;, &agr;-branched carboxylic acids 失效
标题翻译：制备α支链羧酸的方法
公开(公告)号：US06211406B1
公开(公告)日：2001-04-03
申请号：US09421727
申请日：1999-10-20
申请人： Jean-Paul Lange , Vincent Otten , Hans Arie Stil
发明人： Jean-Paul Lange , Vincent Otten , Hans Arie Stil
IPC分类号： C07C5114
CPC分类号： C07C51/12 , C07C51/14 , C07C53/128
摘要： A process for manufacture of &agr;,&agr;-branched carboxylic acids from linear olefins by means of reaction with carbon monoxide and an acid catalyst, characterized in that a linear olefin containing from 2 to 5 carbon atoms, or a precursor thereof, is reacted in a batch reactor or a continuous reactor, with carbon monoxide and water, in the presence of a catalyst having sufficient acid groups to provide requisite protons for the formation of Koch acid, and in the presence of a polar non-coordinating organic solvent.
摘要翻译：一种通过与一氧化碳和一种酸催化剂的反应由直链烯烃制备α，α-支链羧酸的方法，其特征在于含有2至5个碳原子的直链烯烃或其前体在在具有足够酸基的催化剂存在下，使用一氧化碳和水的连续反应器，以提供用于形成科赫酸的必需质子，并在极性非配位有机溶剂的存在下进行。

34. 发明授权

US08372164B2 Gasoline composition and process for the preparation of alkylfurfuryl ether 有权
标题翻译：汽油组成和制备烷基糠醚的方法
公开(公告)号：US08372164B2
公开(公告)日：2013-02-12
申请号：US12808722
申请日：2008-12-18
申请人： Rene Johan Haan , Jean-Paul Lange
发明人： Rene Johan Haan , Jean-Paul Lange
IPC分类号： C10L1/18
CPC分类号： C10L1/023 , C10L1/14 , C10L1/1824 , C10L1/1855 , C10L1/19 , C10L10/10
摘要： A gasoline composition containing in the range of from 0.1 to 30 wt % alkylfurfuryl ether with an alkyl group having 1 to 4 carbon atoms is provided. The gasoline composition is prepared by blending the alkylfurfuryl ether in a gasoline base fuel. The alkylfurfuryl ether is prepared by reacting an alkyl alcohol having in the range of 1 to 4 carbon atoms is reacted with furfuryl alcohol by contacting a liquid phase comprising the alkyl alcohol and furfuryl alcohol with an acidic zeolite catalyst at a temperature in the range of from 50 to 200° C.
摘要翻译：提供含有0.1至30重量％烷基糠醚与具有1至4个碳原子的烷基的汽油组合物。通过将烷基糠醚混合在汽油基础燃料中制备汽油组合物。烷基糠醚通过使具有1至4个碳原子的烷基醇与糠醇反应来制备，通过使含有烷基醇和糠醇的液相与酸性沸石催化剂接触，其温度范围为 50〜200℃

35. 发明申请

US20110041792A1 GASOLINE COMPOSITIONS 有权
标题翻译：汽油组合物
公开(公告)号：US20110041792A1
公开(公告)日：2011-02-24
申请号：US12787261
申请日：2010-05-25
申请人： Allison FELIX-MOORE , Jean-Paul Lange , Johanne Smith
发明人： Allison FELIX-MOORE , Jean-Paul Lange , Johanne Smith
IPC分类号： F02B43/00 , C10L1/19
CPC分类号： C10L10/08 , C10L1/023 , C10L1/19 , C10L10/10
摘要： An unleaded gasoline composition comprising: (i) a gasoline base fuel; and (ii) component A, wherein component A is an alkyl alkenoate compound, or a mixture of alkyl alkenoate compounds, selected from compounds of formula I: wherein R1 is a linear alkenyl group containing 3 to 5 carbon atoms, optionally substituted by a methyl group, and R2 is a linear or branched alkyl group containing 1 to 6 carbon atoms.The gasoline composition of the present invention exhibits good lubricity. The gasoline composition of the invention in another aspect provides increased sensitivity.
摘要翻译：一种无铅汽油组合物，包括：（i）汽油基燃料; 和（ii）组分A，其中组分A是烷基烯酸酯化合物或选自式I化合物的烷基烯酸酯化合物的混合物：其中R 1是含有3至5个碳原子的直链烯基，任选被甲基基团，R2是含有1至6个碳原子的直链或支链烷基。本发明的汽油组合物表现出良好的润滑性。本发明的另一方面的汽油组合物提供了增加的灵敏度。

36. 发明申请

US20100292507A1 PROCESS FOR CONVERTING LEVULINIC ACID INTO PENTANOIC ACIDITLE 审中-公开
标题翻译：将维生素酸转化成苦味酸的方法
公开(公告)号：US20100292507A1
公开(公告)日：2010-11-18
申请号：US12668715
申请日：2008-07-09
申请人： Jean-Paul Lange
发明人： Jean-Paul Lange
IPC分类号： C07C53/00
CPC分类号： C07C51/377 , C07C53/126
摘要： A process for converting levulinic acid into pentanoic acid, comprising the following steps: (a) supplying hydrogen and a feedstock comprising levulinic acid to a first catalytic zone comprising a strongly acidic catalyst and a hydrogenation metal; (b) converting, in the first catalytic zone, the levulinic acid at a temperature in the range of from 100 to 250° C. into gamma valerolactone to obtain a first effluent comprising gamma valerolactone; (c) supplying at least part of the first effluent to a second catalytic zone comprising a strongly acidic catalyst and a hydrogenation metal; and (d) converting, in the second catalytic zone, gamma valerolactone into pentanoic acid at a temperature in the range of from 200 to 350° C. to obtain a second effluent comprising pentanoic acid, wherein the conversion temperature in the first catalytic zone is lower than the conversion temperature in the second catalytic zone, and wherein the acidic catalyst and the hydrogenation metal in the first catalytic zone has the same composition as the acidic catalyst and the hydrogenation metal in the second catalytic zone.
摘要翻译：一种将乙酰丙酸转化为戊酸的方法，包括以下步骤：（a）向包含强酸性催化剂和氢化金属的第一催化区供应氢和包含乙酰丙酸的原料; （b）在第一催化区中将乙酰丙酸在100-250℃的温度范围内转化成γ-戊内酯，得到含有γ-戊内酯的第一流出液; （c）将至少部分第一流出物供应到包含强酸性催化剂和氢化金属的第二催化区; 和（d）在第二催化区域中将γ-戊内酯在200-350℃的温度范围内转化成戊酸，得到包含戊酸的第二流出物，其中第一催化区域中的转化温度为低于第二催化区中的转化温度，并且其中第一催化区中的酸性催化剂和氢化金属具有与酸性催化剂和第二催化区中的氢化金属相同的组成。

37. 发明申请

US20070142664A1 Process for the preparation of an alkyl alkenoate 审中-公开
标题翻译：制备烷基链烯酸酯的方法
公开(公告)号：US20070142664A1
公开(公告)日：2007-06-21
申请号：US10583059
申请日：2004-12-16
申请人： Rene Haan , Jean-Paul Lange
发明人： Rene Haan , Jean-Paul Lange
IPC分类号： C07C69/52
CPC分类号： C07C67/03 , C07C69/533
摘要： A process for the preparation of an alkyl alkenoate, wherein a lactone of the general molecular formula (I) wherein n is 1, 2 or 3, R1 is a C1-C4 alkyl group, and R2, R3 and R4 are, independently, a H atom or a C1-C4 alkyl group, is reacted with a C1-C4 alkyl alcohol in a liquid phase in the presence of a strong acid catalyst at transesterification conditions to form the alkyl alkenoate, wherein alkyl alkenoate and alcohol are continuously removed from the liquid phase by distillation.
摘要翻译：一种制备烷基链烯酸酯的方法，其中通式（I）的内酯，其中n为1,2或3，R 1为C 1〜 -C 4烷基，R 2，R 3和R 4独立地是H原子或C 1 -C 4烷基与C 1 -C 4烷基醇反应，得到C 1 -C 4 - 在酯交换条件下在强酸催化剂存在下的液相以形成烷基链烯酸酯，其中烷基链烯酸酯和醇通过蒸馏从液相中连续除去。

38. 发明申请

US20070049771A1 PROCESS FOR THE CONVERSION OF FURFURYL ALCOHOL INTO LEVULINIC ACID OR ALKYL LEVULINATE 失效
标题翻译：将呋喃酒精转化为橄榄酸或碱性橄榄油的方法
公开(公告)号：US20070049771A1
公开(公告)日：2007-03-01
申请号：US11466630
申请日：2006-08-23
申请人： Wouter Van De Graaf , Jean-Paul Lange
发明人： Wouter Van De Graaf , Jean-Paul Lange
IPC分类号： C07C59/76
CPC分类号： C07C51/00 , C07C67/00 , C07C59/185 , C07C69/716
摘要： A process for the conversion of furfuryl alcohol into levulinic acid or alkyl levulinate comprising contacting furfuryl alcohol and water or an alkyl alcohol with a porous heterogeneous catalyst comprising strong acid ion-exchange resin, wherein the catalyst has pores with an average pore diameter in the range of from 1 to 1000 nm.
摘要翻译：一种将糠醇转化成乙酰丙酸或乙酰丙酸烷基酯的方法，包括使糠醇与水或烷基醇与包含强酸离子交换树脂的多孔非均相催化剂接触，其中催化剂具有平均孔径在该范围内的孔为1〜1000nm。

39. 发明申请

US20060162239A1 Process for the hydrogenation of a lactone or of a carboxylic acid or an ester having a gamma-carbonyl group 有权
标题翻译：内酯或具有γ-羰基的羧酸或酯的氢化方法
公开(公告)号：US20060162239A1
公开(公告)日：2006-07-27
申请号：US11314404
申请日：2005-12-21
申请人： Peter Van Den Brink , Klaas Von Hebel , Jean-Paul Lange , Leonardus Petrus
发明人： Peter Van Den Brink , Klaas Von Hebel , Jean-Paul Lange , Leonardus Petrus
IPC分类号： C10L1/18 , C07C69/02
CPC分类号： C07C51/377 , C07C53/126
摘要： The invention provides a process for the hydrogenation of a reactant selected from the group consisting of: (a) a 5- or 6-membered lactone that is substituted at the ring-closing carbon atom and has a proton at a carbon atom adjacent to the ring-closing carbon atom; (b) an ester of a carboxylic acid having a gamma-carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group; and (c) a carboxylic acid having a gamma-carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group, wherein the reactant is contacted with a strongly acidic heterogeneous catalyst comprising a hydrogenating metal, in the presence of hydrogen, at a temperature in the range of from 100 to 350° C. and a pressure in the range of from 1 to 150 bar (absolute). The invention further provides a fuel composition, preferably a diesel composition, comprising di-alkyl 4-methylnonanedioate or di-alkyl 3-ethyl-4-methylheptanedioate.
摘要翻译：本发明提供了一种用于氢化反应物的方法，所述反应物选自：（a）在闭环碳原子处被取代并且在与碳原子相邻的碳原子处具有质子的5-或6-元内酯闭环碳原子; （b）在与羰基的碳原子相邻的碳原子处具有γ-羰基和质子的羧酸的酯; 和（c）在与羰基的碳原子相邻的碳原子处具有γ-羰基和质子的羧酸，其中反应物与包含氢化金属的强酸性多相催化剂在存在下，氢气，温度范围为100至350℃，压力范围为1至150巴（绝对）。本发明还提供一种燃料组合物，优选含有4-甲基壬二酸二烷基酯或3-乙基-4-甲基庚二酸二烷基酯的柴油组合物。

40. 发明申请

US20050148787A1 Process for the preparation of propylene carbonate 审中-公开
标题翻译：碳酸丙烯酯的制备方法
公开(公告)号：US20050148787A1
公开(公告)日：2005-07-07
申请号：US10994741
申请日：2004-11-22
申请人： Johannes Gerhardus Beckers , Evert Heide , Gerardus Martinus Van Kessel , Jean-Paul Lange
发明人： Johannes Gerhardus Beckers , Evert Heide , Gerardus Martinus Van Kessel , Jean-Paul Lange
IPC分类号： C07C29/12 , C07C68/06 , C07D317/36 , C07C69/96
CPC分类号： C07C29/12 , C07C68/065 , C07D317/36 , C07C69/96 , C07C31/205
摘要： The invention is related to a process involving contacting a propylene oxide feed with carbon dioxide in the presence of a suitable catalyst to obtain a reaction mixture containing propylene carbonate in which process the propylene oxide feed contains at least 50 ppmw of acids and/or carbonyls.
摘要翻译：本发明涉及涉及使环氧丙烷进料与二氧化碳在合适的催化剂存在下接触以获得含有碳酸丙烯酯的反应混合物的方法，其中环氧丙烷进料含有至少50ppmw的酸和/或羰基。

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