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21. 发明申请

WO2015068095A1 STEREOREGULAR DIBLOCK POLYBUTADIENES HAVING A 1,4-CIS/SYNDIOTACTIC 1,2 STRUCTURE FROM STEREOSPECIFIC POLYMERIZATION 审中-公开
标题翻译：具有1,4- CIS / SYNDIOTACTIC 1,2结构的立体双嵌段聚丁二烯由立体异构聚合
公开(公告)号：WO2015068095A1
公开(公告)日：2015-05-14
申请号：PCT/IB2014/065768
申请日：2014-11-03
申请人： VERSALIS S.P.A.
发明人： MASI, Francesco , SOMMAZZI, Anna , RICCI, Giovanni , LEONE, Giuseppe , COPPOLA, Salvatore
IPC分类号： C08F295/00 , C08F4/655
CPC分类号： C08F295/00 , C08F4/7006 , C08F4/7008 , C08F4/7042 , C08F4/7044
摘要： Stereoregular diblock polybutadiene composed of a polybutadiene block having a 1,4-cis structure and a polybutadiene block having a syndiotactic 1,2 structure. Said stereoregular diblock polybutadiene can be advantageously used in both the footwear industry (for example, in the production of soles for shoes) and in the production of tires for motor vehicles and/or trucks.
摘要翻译：由具有1,4-顺式结构的聚丁二烯嵌段和具有间同立构1,2结构的聚丁二烯嵌段组成的立体规整性二嵌段聚丁二烯。所述有规立构双嵌段聚丁二烯可有利地用于鞋类工业（例如用于制鞋的鞋底）和用于机动车辆和/或卡车的轮胎的生产中。

22. 发明申请

WO2014097245A1 PROCESS FOR THE PREPARATION OF (CO) POLYMERS OF CONJUGATED DIENES IN THE PRESENCE OF A CATALYTIC SYSTEM COMPRISING A BIS-IMINO-PYRIDINE COMPLEX OF COBALT 审中-公开
标题翻译：在含有BIS-IMINO-吡啶复合物的催化体系存在下制备（CO）聚合物的方法
公开(公告)号：WO2014097245A1
公开(公告)日：2014-06-26
申请号：PCT/IB2013/061193
申请日：2013-12-20
申请人： VERSALIS S.P.A.
发明人： MASI, Francesco , RICCI, Giovanni , SOMMAZZI, Anna , LEONE, Giuseppe , CALDARARO, Maria
IPC分类号： C08F36/06 , C08F136/06
CPC分类号： C08F136/06 , C07F15/065 , C08F4/7096 , C08F36/06 , C08F4/7042
摘要： Process for the preparation of (co) polymers of conjugated dienes which comprises polymerizing at least one conjugated diene in the presence of a catalytic system comprising at least one bis-imino-pyridine complex of cobalt having general formula (I) : wherein : R 2 and R 3 , equal to or different from each other, represent a hydrogen atom; or they are selected from linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups, optionally halogenated, cycloalkyl groups optionally substituted, aryl groups optionally substituted; R 1 and R 4 , different from each other, represent a hydrogen atom; or they are selected from linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups, optionally halogenated, cycloalkyl groups optionally substituted, aryl groups optionally substituted; arylalkyl groups; or R 1 and R 2 can be optionally bound to each other to form, together with the other atoms to which they are bound, a cycle containing from 3 to 6 carbon atoms, saturated, unsaturated, or aromatic, optionally substituted with linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, said cycle optionally containing other heteroatoms such as, for example, oxygen, sulfur, nitrogen, silicon, phosphorous, selenium; or R 3 and R 4 , can be optionally bound to each other to form, together with the other atoms to which they are bound, a cycle containing from 3 to 6 carbon atoms, saturated, unsaturated, or aromatic, optionally substituted with linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, said cycle optionally containing other heteroatoms such as, for example, oxygen, sulfur, nitrogen, silicon, phosphorous, selenium; R 5 , R 6 and R 7 , equal to or different from each other, represent a hydrogen atom, or they are selected from linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, optionally halogenated, cycloalkyl groups optionally substituted; aryl groups optionally substituted; arylalkyl groups; or R 5 and R 6 , can be optionally bound to each other to form, together with the other atoms to which they are bound, a cycle containing from 3 to 6 carbon atoms, saturated, unsaturated, or aromatic, optionally substituted with linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, said cycle optionally containing other heteroatoms such as, for example, oxygen, -sulfur, nitrogen, silicon, phosphorous, selenium; or R 6 and R 7 , can be optionally bound to each other to form, together with the other atoms to which they are bound, a cycle containing from 3 to 6 carbon atoms, saturated, unsaturated, or aromatic, optionally substituted with linear or branched C 1 - C 20 , preferably C 1 -C 15 , alkyl groups, said cycle optionally containing other heteroatoms such as, for example, oxygen, sulfur, nitrogen, silicon, phosphorous, selenium; X 1 and X 2 , equal to or different from each other, represent a halogen atom such as, for example, chlorine, bromine, iodine; or they are selected from linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, -OCOR 8 groups or -OR 8 groups wherein R 8 is selected from linear or branched C 1 -C 20 / preferably C 1 -C 15 , alkyl groups.
摘要翻译：制备共轭二烯的（共）聚合物的方法，其包括在包含至少一种具有通式（I）的钴的二亚氨基 - 吡啶络合物的催化体系存在下聚合至少一种共轭二烯：其中：R2和 R 3彼此相同或不同，表示氢原子; 或者它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，任选卤代的环烷基，任选取代的芳基，任选取代的芳基; R1和R4彼此不同，表示氢原子; 或者它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，任选卤代的环烷基，任选取代的芳基，任选取代的芳基; 芳基烷基; 或者R 1和R 2可以任选地彼此结合形成与其结合的其它原子一起，含有3至6个碳原子的饱和的，不饱和的或芳族的，任选地被直链或支链C1- C20，优选C1-C15烷基，所述循环任选地含有其它杂原子，例如氧，硫，氮，硅，磷，硒; 或R 3和R 4可以任选地彼此结合形成与它们所结合的其它原子一起形成含有3-6个碳原子的饱和的，不饱和的或芳族的，任选被直链或支链C1 -C 20，优选C 1 -C 15烷基，所述循环任选地含有其它杂原子，例如氧，硫，氮，硅，磷，硒; R 5，R 6和R 7彼此相同或不同，表示氢原子，或它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，任选卤代的环烷基任选取代; 任选取代的芳基; 芳基烷基; 或者R 5和R 6可以任选地彼此结合形成与它们所连接的其它原子一起形成含有3-6个碳原子的饱和的，不饱和的或芳族的，任选被直链或支链C1 -C 20，优选C 1 -C 15烷基，所述循环任选地含有其它杂原子，例如氧，硫，氮，硅，磷，硒; 或R6和R7可以任选地彼此结合形成与其结合的其它原子一起，含有3至6个碳原子的饱和，不饱和或芳族的环，任选被直链或支链C1 -C 20，优选C 1 -C 15烷基，所述循环任选地含有其它杂原子，例如氧，硫，氮，硅，磷，硒; X 1和X 2彼此相同或不同，表示卤素原子，例如氯，溴，碘; 或者它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，-OCOR 8基团或-OR 8基团，其中R 8选自直链或支链C 1 -C 20，优选C 1 -C 15烷基。

23. 发明申请

WO2014097087A1 PROCESS FOR THE PREPARATION OF (CO)POLYMERS OF CONJUGATED DIENES IN THE PRESENCE OF A CATALYTIC SYSTEM COMPRISING AN OXO-NITROGENATED COMPLEX OF COBALT 审中-公开
标题翻译：在含有氧化复合物的催化体系中存在共聚二烯的（CO）聚合物的方法
公开(公告)号：WO2014097087A1
公开(公告)日：2014-06-26
申请号：PCT/IB2013/060905
申请日：2013-12-13
申请人： VERSALIS S.P.A
发明人： RICCI, Giovanni , LEONE, Giuseppe , SOMMAZZI, Anna , MASI, Francesco
IPC分类号： C08F136/06
CPC分类号： C08F136/06 , C08F4/704 , C08F4/7044 , C08F36/04 , C08F36/06
摘要： Process for the preparation of (co) polymers of conjugated dienes which comprises polymerizing at least one conjugated diene in the presence of a catalytic system comprising at least one oxo-nitrogenated complex of cobalt having general formula (I),wherein : - R 1 and R 2 , equal to or different from each other, represent a hydrogen atom; or they are selected from linear or branched C 1 -C 20 , preferably C 1 -C 15 , alkyl groups, optionally halogenated; cycloalkyl groups optionally substituted; aryl groups optionally substituted; - Y represents an oxygen atom; or a group -N-R 3 wherein R 3 represents a hydrogen atom, or it is selected from linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups, optionally halogenated, cycloalkyl groups optionally substituted-; aryl groups optionally substituted; or, when Y represents a group -N-R 3 , R 2 and R 3 can be optionally bound to each other to form, together with the other atoms to which they are bound, a cycle containing from 3 to 6 carbon atoms, saturated, unsaturated, or aromatic, optionally substituted with linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups, said cycle optionally containing heteroatoms such as, for example, oxygen, sulfur, nitrogen, silicon, phosphorous, selenium; - X 1 and X 2 , equal to or different from each other, represent a halogen atom such as, for example, chlorine, bromine, iodine; or they are selected from linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups, -OCOR 4 groups or -OR 4 groups wherein R 4 is selected from linear or branched C 1 -C 20 preferably C 1 -C 15 , alkyl groups.
摘要翻译：制备共轭二烯的（共）聚合物的方法，其包括在催化体系的存在下聚合至少一种共轭二烯，所述催化体系包含至少一个通式（I）的含氧的含氮复合物的钴，其中：-R 1和R 2 相同或不同，表示氢原子; 或者它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，任选卤代; 任选取代的环烷基; 任选取代的芳基; -Y表示氧原子; 或其中R 3表示氢原子的基团-N-R 3，或其选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，任选卤代的环烷基，任选取代的; 任选取代的芳基; 或者当Y代表基团-N-R 3时，R 2和R 3可以彼此结合，形成与其结合的其它原子一起含有3至6个碳原子的饱和的，不饱和的，或芳族的，任选地被直链或支链的C 1 -C 20，优选C 1 -C 15烷基取代，所述循环任选地含有杂原子，例如氧，硫，氮，硅，磷，硒; -X 1和X 2彼此相同或不同，表示卤素原子，例如氯，溴，碘; 或者它们选自直链或支链C 1 -C 20，优选C 1 -C 15烷基，-OCOR 4基团或-OR 4基团，其中R 4选自直链或支链C 1 -C 20，优选C 1 -C 15烷基。

24. 发明申请

WO2013037913A1 BIS-IMINE PYRIDINE COMPLEX OF LANTHANIDES, CATALYTIC SYSTEM COMPRISING SAID BIS-IMINE PYRIDINE COMPLEX AND PROCESS FOR THE (CO)POLYMERIZATION OF CONJUGATED DIENES 审中-公开
标题翻译：双胺双膦酸复合物，包含双相异构体吡啶复合物的催化体系和共聚二烯的（CO）聚合方法
公开(公告)号：WO2013037913A1
公开(公告)日：2013-03-21
申请号：PCT/EP2012/067992
申请日：2012-09-13
申请人： VERSALIS S.P.A. , RICCI, Giovanni , SOMMAZZI, Anna , LEONE, Giuseppe , BOGLIA, Aldo , MASI, Francesco , CALDARARO,, Maria
发明人： RICCI, Giovanni , SOMMAZZI, Anna , LEONE, Giuseppe , BOGLIA, Aldo , MASI, Francesco , CALDARARO,, Maria
IPC分类号： C08F4/68 , C08F36/04 , C08F136/06
CPC分类号： C08F36/08 , C08F36/00 , C08F36/04 , C08F36/06 , C08F136/00 , C08F2410/04 , C08F4/545
摘要： A bis-imine pyridine complex of lanthanides having general formula (I): Said bis-imine pyridine complex of lanthanides having general formula (I) can be advantageously used in a catalytic system for the (co)polymerization of conjugated dienes.
摘要翻译：具有通式（I）的镧系元素的双亚胺吡啶络合物：具有通式（I）的镧系元素的所述双亚胺吡啶络合物可有利地用于共轭二烯（共）聚合的催化体系中。

25. 发明授权

EP2658860B1 METAL ALKYL-ARENES AND PROCESSES FOR THE PREPARATION THEREOF 有权
标题翻译：金属烷基 - 芳香族化合物及其制备方法
公开(公告)号：EP2658860B1
公开(公告)日：2017-12-13
申请号：EP11805043.4
申请日：2011-12-23
申请人： Versalis S.p.A.
发明人： PAMPALONI, Guido , RENILI, Filippo , SOMMAZZI, Anna , MARCHETTI, Fabio , MASI, Francesco , POLESELLO, Mario
IPC分类号： C07F7/00
CPC分类号： C07F19/00 , B01J31/122 , C07F7/006 , C08F4/42 , C08F10/00 , C08F4/659

26. 发明公开

EP3186290A1 SOLID CATALYST FOR THE (CO)POLYMERISATION OF -OLEFINS AND PROCESS FOR THE PREPARATION THEREOF 有权转让
标题翻译：烯烃（共）聚合用固体催化剂及其制备方法
公开(公告)号：EP3186290A1
公开(公告)日：2017-07-05
申请号：EP15752947.0
申请日：2015-07-30
申请人： Versalis S.p.A
发明人： MASI, Francesco , SOMMAZZI, Anna , POLESELLO, Mario
IPC分类号： C08F210/16 , C08F4/655
摘要： An improved solid Ziegler-Natta type catalyst for the (co)polymerisation of ethylene and α-olefins, particularly in high-temperature processes, such as for example adiabatic solution processes and high-pressure adiabatic processes with elevated productivity, is provided. Said catalyst is obtained by means of an original process comprising dissolving in hydrocarbons, compounds of titanium, magnesium and optionally a metal selected from hafnium and zirconium, and reprecipitating them in two steps in succession, the first of which is chlorination and the second reduction.
摘要翻译：提供了用于乙烯和α-烯烃（共）聚合的改进的固体齐格勒 - 纳塔型催化剂，特别是在高温过程中，例如绝热溶液过程和具有高生产率的高压绝热过程。所述催化剂通过包括溶于烃，钛，镁和任选的选自铪和锆的金属的化合物的原始方法获得，并且连续两步再沉淀它们，其中第一步是氯化和第二次还原。

27. 发明公开

EP3066140A1 STEREOREGULAR DIBLOCK POLYBUTADIENES HAVING A 1,4-CIS/SYNDIOTACTIC 1,2 STRUCTURE FROM STEREOSPECIFIC POLYMERIZATION 有权
标题翻译：具有1,4- CIS / SYNDIOTACTIC 1,2结构的立体双嵌段聚丁二烯由立体异构聚合
公开(公告)号：EP3066140A1
公开(公告)日：2016-09-14
申请号：EP14812613.9
申请日：2014-11-03
申请人： Versalis S.p.A.
发明人： MASI, Francesco , SOMMAZZI, Anna , RICCI, Giovanni , LEONE, Giuseppe , COPPOLA, Salvatore
IPC分类号： C08F295/00 , C08F4/655
CPC分类号： C08F295/00 , C08F4/7006 , C08F4/7008 , C08F4/7042 , C08F4/7044
摘要： Stereoregular diblock polybutadiene composed of a polybutadiene block having a 1,4-cis structure and a polybutadiene block having a syndiotactic 1,2 structure. Said stereoregular diblock polybutadiene can be advantageously used in both the footwear industry (for example, in the production of soles for shoes) and in the production of tires for motor vehicles and/or trucks.
摘要翻译：由具有1,4-顺式结构的聚丁二烯嵌段和具有间同立构1,2结构的聚丁二烯嵌段构成的立体规则性二嵌段聚丁二烯。所述有规立构双嵌段聚丁二烯可有利地用于鞋类工业（例如用于制鞋的鞋底）以及用于机动车辆和/或卡车的轮胎的生产。

28. 发明授权

EP2504366B1 CATALYSTS OF THE ZIEGLER-NATTA TYPE FOR THE (CO)POLYMERIZATION OF -OLEFINS WITH A HIGH PRODUCTIVITY 有权
标题翻译：齐格勒 - 纳塔催化剂用于以高生产率的烯烃的（共）聚合
公开(公告)号：EP2504366B1
公开(公告)日：2014-07-30
申请号：EP10784264.3
申请日：2010-11-18
申请人： versalis S.p.A.
发明人： MASI, Francesco , POLESELLO, Mario , FUSCO, Roberto , SOMMAZZI, Anna , PROTO, Antonio Alfonso , MEDA, Laura , CONTI, Giuseppe , MENCONI, Francesco
IPC分类号： C08F4/655 , C08F10/00
CPC分类号： C08F10/00 , C08F210/16 , C08F2410/03 , C08F4/6557 , C08F210/14 , C08F2500/12

29. 发明公开

EP2658860A1 METAL ALKYL-ARENES AND PROCESSES FOR THE PREPARATION THEREOF 有权
标题翻译： METALLALKYLARENE UND VERFAHREN ZU IHRER HERSTELLUNG
公开(公告)号：EP2658860A1
公开(公告)日：2013-11-06
申请号：EP11805043.4
申请日：2011-12-23
申请人： Versalis S.p.A.
发明人： PAMPALONI, Guido , RENILI, Filippo , SOMMAZZI, Anna , MARCHETTI, Fabio , MASI, Francesco , POLESELLO, Mario
IPC分类号： C07F7/00
CPC分类号： C07F19/00 , B01J31/122 , C07F7/006 , C08F4/42 , C08F10/00 , C08F4/659
摘要： Metal alkyl-arene having general formula (I) or (Ia): M (eta6-arene)2Al1XrRs (I) M (eta6-arene)AlqXrRs (Ia) wherein: -M represents zirconium (Zr), hafnium (Hf), or mixtures thereof, preferably zirconium; -arene represents a benzene, or a benzene 10 substituted with from 1 to 6 linear or branched C1-C6 alkyl groups, or mixtures thereof; -X represents a halogen atom selected from chlorine, bromine, fluorine, iodine, preferably chlorine; -R represents a linear or branched C1-C15 alkyl group; -q is a number ranging from 2 to 6, preferably 3 for a metal alkyl-arene having general formula (I), 2 for a metal alkyl-arene having general formula (Ia); -r is a number ranging from 1 to 20, preferably 9 for a metal alkyl-arene having general formula (I), 6 for a metal alkyl-arene having general formula (Ia); -s is a number ranging from 1 to 6, preferably 2. Said metal alkyl-arene can be advantageously used for the preparation of solid components of catalysts for the (co)polymerization of alpha-olefins.
摘要翻译：具有通式（I）或（Ia）的金属烷基芳烃：M（＆eegr。6-芳烃）2AlqXrRs（I）M（＆eegr; 6-芳烃）AlqXrRs（Ia）其中：-M代表锆（Zr），铪（Hf），或其混合物，优选锆; 芳烃代表苯或被1至6个直链或支链C 1 -C 6烷基取代的苯10，或其混合物; -X表示选自氯，溴，氟，碘，优选氯的卤素原子; -R表示直链或支链的C 1 -C 15烷基; 对于具有通式（I）的金属烷基芳烃，对于具有通式（Ia）的金属烷基芳烃，-q为2至6的数，优选3。对于具有通式（I）的金属烷基芳烃，对于具有通式（Ia）的金属烷基芳烃，-r为1至20的数，优选9。 -s是1至6的数，优选2.所述金属烷基芳烃可有利地用于制备用于α-烯烃（共）聚合的催化剂的固体组分。

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