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21. 发明授权

US08021864B2 Biomass-resource-derived polyester and production process thereof 有权
公开(公告)号：US08021864B2
公开(公告)日：2011-09-20
申请号：US12858046
申请日：2010-08-17
申请人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
发明人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
IPC分类号： C12P7/48
CPC分类号： C08G63/16 , C08G63/20 , C08G63/78 , C08L1/00 , C08L3/00 , C08L5/00 , C08L67/02 , C08L99/00 , C08L2201/06 , C08L2666/02
摘要： The present invention provides a resin capable of contributing greatly to solve environmental problems and problems related to exhaustion of fossil fuel resources and having physical properties suited for practical use.The polyester according to the present invention has a diol and a dicarboxylic acid as constituent components and has an amount of terminal acid of 50 equivalents/metric ton or less.

22. 发明申请

US20060293492A1 Process for producing aliphatic polyester, a polyester produced by the process, and an aliphatic polyester 审中-公开
标题翻译：制造脂肪族聚酯的方法，通过该方法制造的聚酯和脂肪族聚酯
公开(公告)号：US20060293492A1
公开(公告)日：2006-12-28
申请号：US11376418
申请日：2006-03-16
申请人： Takayuki Aoshima , Toyomasa Hoshino , Hitoshi Nimura
发明人： Takayuki Aoshima , Toyomasa Hoshino , Hitoshi Nimura
IPC分类号： C08G63/00
CPC分类号： C08G63/82
摘要： An aliphatic polyester with a high polymerization degree having an excellent thermal stability is produced by reacting diol unit(s) and aliphatic dicarboxylic acid unit(s) in the presence of a catalyst comprising a metal oxide containing at least one element from the group consisting of metal elements belonging to the Groups 3 to 6 of the Periodic Table and at least one element selected from the group consisting of a silicon element and a metal element from Groups 1, 2, 12, 13, and 14 of the Periodic Table in an industrially advantageous process.
摘要翻译：通过使二醇单元和脂肪族二羧酸单元在包含含有至少一种元素的金属氧化物的催化剂的存在下反应制备具有优异热稳定性的脂族聚酯，所述催化剂包含至少一种元素，属于元素周期表第3至6族的金属元素和选自元素周期表第1,2,12,13和14族的元素和金属元素中的至少一种元素在工业上有利的过程。

23. 发明授权

US10287393B2 Biomass-resource-derived polyester and production process thereof 有权
公开(公告)号：US10287393B2
公开(公告)日：2019-05-14
申请号：US15693646
申请日：2017-09-01
申请人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
发明人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
IPC分类号： C08G63/16 , C08G63/20 , C08G63/78 , C08L67/02 , C08L1/00 , C08L3/00 , C08L5/00 , C08L99/00
摘要： An aliphatic dicarboxylic acid, an aliphatic diol or a derivatives thereof and/or as succinic acid, a butane diol, or a both-hydroxy-terminated polyether having the number of carbon atoms of 4 to 1000, each of which is derived from a biomass resource and has nitrogen atoms in an amount of 0.01 to 100 ppm. Products and methods using these materials are also provided.

24. 发明授权

US07888084B2 Biomass-resource-derived polyester and production process thereof 有权
公开(公告)号：US07888084B2
公开(公告)日：2011-02-15
申请号：US11912212
申请日：2006-04-21
申请人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
发明人： Takayuki Aoshima , Yasuaki Miki , Katsuhisa Kumazawa , Satoshi Katou , Tadashi Uyeda , Toyomasa Hoshino , Noboru Shintani , Kenji Yamagishi , Atsushi Isotani
IPC分类号： C12P7/48
摘要： The present invention provides a resin capable of contributing greatly to solve environmental problems and problems related to exhaustion of fossil fuel resources and having physical properties suited for practical use.The polyester according to the present invention has a diol and a dicarboxylic acid as constituent components and has an amount of terminal acid of 50 equivalents/metric ton or less.

25. 发明授权

US07317069B2 Aliphatic polyester and process for producing the same 有权
标题翻译：脂肪族聚酯及其制造方法
公开(公告)号：US07317069B2
公开(公告)日：2008-01-08
申请号：US11282622
申请日：2005-11-21
申请人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
发明人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
IPC分类号： C08G63/00 , C08G63/12 , C08G63/16 , C08K3/00 , C08F2/44 , C08F2/00
CPC分类号： C08G63/78 , C08G63/16
摘要： An object of the present invention is to provide an aliphatic polyester which is produced as a high-molecular-weight one without using a chain extender such as an isocyanate compound or a carbonate compound and is excellent in moldability in injection molding, blow molding, or extrusion molding, thermal stability, and mechanical properties such as tensile properties.The invention relates to an aliphatic polyester comprising an aliphatic diol unit, an aliphatic dicarboxylic acid unit, and a unit of an organic acid having a pKa value of 3.7 or below at 25° C., wherein a content of a carbonate bond contained in the polyester is less than 1 mol %, a content of a urethane bond is less than 0.06 mol %, a content of an aliphatic monooxymonocarboxylic acid unit is less than 0.02 mol %, a content of the phosphorus atom derived from a phosphorus compound selected from among organic phosphinic acids, organic phosphonic acids, and hydrogen phosphate salts is less than 10−9 mol %, based on the whole monomer units constituting the polyester, and a reduced viscosity (ηsp/C) is 1.6 or more.
摘要翻译：本发明的目的是提供一种不使用异氰酸酯化合物或碳酸酯化合物等增链剂作为高分子量制造的脂肪族聚酯，并且在注射成型，吹塑成型或挤出成型，热稳定性和机械性能如拉伸性能。本发明涉及包含脂肪族二醇单元，脂肪族二羧酸单元和25℃下pKa值为3.7以下的有机酸单元的脂肪族聚酯，其中，所含有的碳酸酯键的含量聚酯小于1摩尔％，氨基甲酸酯键的含量小于0.06摩尔％，脂族单氧基单羧酸单元的含量小于0.02摩尔％，磷化合物的磷原子的含量选自基于构成聚酯的全部单体单元，有机次膦酸，有机膦酸和磷酸氢盐的含量小于10〜9摩尔％，并且粘度降低（etasp / C）为1.6或更多。

26. 发明授权

US07312002B2 Lithium secondary cell 有权
标题翻译：锂二次电池
公开(公告)号：US07312002B2
公开(公告)日：2007-12-25
申请号：US11047778
申请日：2005-02-02
申请人： Takayuki Aoshima , Iwao Soga , Mitsuharu Kobayashi
发明人： Takayuki Aoshima , Iwao Soga , Mitsuharu Kobayashi
IPC分类号： H01M6/04 , H01M2/14 , H01M4/82 , H01M6/00
CPC分类号： H01M2/22 , H01M2/021 , H01M2/0275 , H01M2/0277 , H01M2/0287 , H01M2/266 , H01M4/525 , H01M6/168 , H01M10/052 , H01M10/0565 , H01M10/0567 , H01M10/0569 , H01M10/4235 , Y10T29/4911
摘要： To improve an impregnation property of an electrolyte and the cycle characteristics, which have been a problem in the case of employing a casing having a variable shape. A lithium secondary cell comprising a casing having a variable shape, and a cell element having a positive electrode, a negative electrode and an electrolyte, sealed in the casing, wherein a compound represented by following formula (1) is contained in the lithium secondary cell: A1-X-A2 (1) (wherein X is a Group VI element in the periodic table, and A1 and A2 represent an aromatic group, provided that A1 and A2 may be the same or different, and may be connected each other to constitute a ring.)
摘要翻译：为了提高电解质的浸渍性和循环特性，在使用具有可变形状的壳体的情况下，这是一个问题。一种锂二次电池，包括具有可变形状的壳体和密封在壳体中的具有正极，负极和电解质的电池元件，其中在锂二次电池中包含下式（1）表示的化合物：<？in-line-formula description =“In-line Formulas”end =“lead”？> A 1 -XA 2（1）<？in-line-formula description =“In-line Formulas”end =“tail “其中X是周期表中的VI族元素，A 1和A 2表示芳族基团，条件是A 1和A 2可以相同或不同，并且可以彼此连接构成环。）

27. 发明申请

US20070093636A1 ALIPHATIC POLYESTER AND PROCESS FOR PRODUCING THE SAME 审中-公开
标题翻译：涤纶涤纶及其制造方法
公开(公告)号：US20070093636A1
公开(公告)日：2007-04-26
申请号：US11613449
申请日：2006-12-20
申请人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
发明人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
IPC分类号： C08G63/02
CPC分类号： C08G63/78 , C08G63/16
摘要： An object of the present invention is to provide an aliphatic polyester which is produced as a high-molecular-weight one without using a chain extender such as an isocyanate compound or a carbonate compound and is excellent in moldability in injection molding, blow molding, or extrusion molding, thermal stability, and mechanical properties such as tensile properties. The invention relates to an aliphatic polyester comprising an aliphatic diol unit, an aliphatic dicarboxylic acid unit, and a unit of an organic acid having a pKa value of 3.7 or below at 25° C., wherein a content of a carbonate bond contained in the polyester is less than 1 mol %, a content of a urethane bond is less than 0.06 mol %, a content of an aliphatic monooxymonocarboxylic acid unit is less than 0.02 mol %, a content of the phosphorus atom derived from a phosphorus compound selected from among organic phosphinic acids, organic phosphonic acids, and hydrogen phosphate salts is less than 10−9 mol %, based on the whole monomer units constituting the polyester, and a reduced viscosity (ηsp/C) is 1.6 or more.
摘要翻译：本发明的目的是提供一种不使用异氰酸酯化合物或碳酸酯化合物等增链剂作为高分子量制造的脂肪族聚酯，并且在注射成型，吹塑成型或挤出成型，热稳定性和机械性能如拉伸性能。本发明涉及包含脂肪族二醇单元，脂肪族二羧酸单元和25℃下pKa值为3.7以下的有机酸单元的脂肪族聚酯，其中，所含有的碳酸酯键的含量聚酯小于1摩尔％，氨基甲酸酯键的含量小于0.06摩尔％，脂族单氧基单羧酸单元的含量小于0.02摩尔％，磷化合物的磷原子的含量选自基于构成聚酯的全部单体单元，有机次膦酸，有机膦酸和磷酸氢盐的含量小于10〜9摩尔％，并且粘度降低（etasp / C）为1.6或更多。

28. 发明申请

US20060155100A1 Aliphatic polyester and process for producing the same 有权
标题翻译：脂肪族聚酯及其制造方法
公开(公告)号：US20060155100A1
公开(公告)日：2006-07-13
申请号：US11282622
申请日：2005-11-21
申请人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
发明人： Takayuki Aoshima , Toyomasa Hoshino , Tadashi Uyeda , Yasuaki Miki
IPC分类号： C08G63/02
CPC分类号： C08G63/78 , C08G63/16
摘要： An object of the present invention is to provide an aliphatic polyester which is produced as a high-molecular-weight one without using a chain extender such as an isocyanate compound or a carbonate compound and is excellent in moldability in injection molding, blow molding, or extrusion molding, thermal stability, and mechanical properties such as tensile properties. The invention relates to an aliphatic polyester comprising an aliphatic diol unit, an aliphatic dicarboxylic acid unit, and a unit of an organic acid having a pKa value of 3.7 or below at 25° C., wherein a content of a carbonate bond contained in the polyester is less than 1 mol %, a content of a urethane bond is less than 0.06 mol %, a content of an aliphatic monooxymonocarboxylic acid unit is less than 0.02 mol %, a content of the phosphorus atom derived from a phosphorus compound selected from among organic phosphinic acids, organic phosphonic acids, and hydrogen phosphate salts is less than 10−9 mol %, based on the whole monomer units constituting the polyester, and a reduced viscosity (ηsp/C) is 1.6 or more.
摘要翻译：本发明的目的是提供一种不使用异氰酸酯化合物或碳酸酯化合物等增链剂作为高分子量制造的脂肪族聚酯，并且在注射成型，吹塑成型或挤出成型，热稳定性和机械性能如拉伸性能。本发明涉及包含脂肪族二醇单元，脂肪族二羧酸单元和25℃下pKa值为3.7以下的有机酸单元的脂肪族聚酯，其中，所含有的碳酸酯键的含量聚酯小于1摩尔％，氨基甲酸酯键的含量小于0.06摩尔％，脂族单氧基单羧酸单元的含量小于0.02摩尔％，磷化合物的磷原子的含量选自基于构成聚酯的全部单体单元，有机次膦酸，有机膦酸和磷酸氢盐的含量小于10〜9摩尔％，并且粘度降低（etasp / C）为1.6或更多。

29. 发明授权

US06340652B1 Catalysts for polymerization of &agr;-olefins, process for producing &agr;-olefin polymers, novel transition metal compounds and catalyst components for polymerization of &agr;-olefin 失效
标题翻译：用于α-烯烃聚合的催化剂，用于生产α-烯烃聚合物的方法，用于α-烯烃聚合的新型过渡金属化合物和催化剂组分
公开(公告)号：US06340652B1
公开(公告)日：2002-01-22
申请号：US08987768
申请日：1997-12-09
申请人： Toshihiko Sugano , Naoshi Iwama , Eiji Isobe , Toru Suzuki , Yasuo Maruyama , Satoshi Hayakawa , Hisashi Shoda , Masami Kashimoto , Taku Kato , Takayuki Aoshima , Sugio Nishimura , Yoshinori Suga , Stefan Sieber
发明人： Toshihiko Sugano , Naoshi Iwama , Eiji Isobe , Toru Suzuki , Yasuo Maruyama , Satoshi Hayakawa , Hisashi Shoda , Masami Kashimoto , Taku Kato , Takayuki Aoshima , Sugio Nishimura , Yoshinori Suga , Stefan Sieber
IPC分类号： B01J3100
CPC分类号： C07F17/00 , C08F4/65912 , C08F4/65916 , C08F4/65927 , C08F110/06 , Y10S526/943 , C08F2500/03 , C08F2500/12 , C08F2500/15
摘要： Catalysts for polymerization of &agr;-olefin, composed of a transition metal compound, an inorganic silicate or an ion exchangeable layer compound other than silicate, and optionally an organoaluminum compound, are described. The transition metal compound is represented by formula (I): where A1 and A2 are each independently a conjugated 5-membered ring ligand, preferably azulene groups, provided that A1 and A2 may be the same or different in a molecule, and at least one of A1 and A2 forms a 7- to 10-membered condensed ring including two adjacent carbon atoms of the conjugated 5-membered ring, which condensed ring is formed by joining two adjacent substitutent groups on the conjugated 5-membered ring; Q is a bridging group of the two conjugated 5-membered rings of A1 and A2 at optional positions of the 5-membered rings; M is a metal atom selected from elements of Group 4-6 of the Periodic Table; and X and Z are each independently a hydrogen atom, a halogen atom, a hydrocarbon group, and amino group, a halogenated hydrocarbon group, an oxygen-containing hydrocarbon group, a nitrogen-containing hydrocarbon group, a phosphorus-containing hydrocarbon group or a silicon-containing hydrocarbon group.
摘要翻译：描述了由过渡金属化合物，无机硅酸盐或除了硅酸盐之外的可离子交换层化合物以及任选的有机铝化合物组成的α-烯烃聚合催化剂。过渡金属化合物由式（I）表示：其中A1和A2各自独立地为共轭五元环配体，优选薁基，条件是A 1和A 2可以在分子中相同或不同，并且至少一个的A1和A2形成包含共轭五元环的两个相邻碳原子的7-至10-元稠环，所述稠合环通过连接共轭五元环上的两个相邻的取代基而形成; Q是在5元环的任选位置的A1和A2的两个共轭五元环的桥连基团; M是选自元素周期表第4-6组元素的金属原子; X和Z各自独立地为氢原子，卤素原子，烃基和氨基，卤代烃基，含氧烃基，含氮烃基，含磷烃基或含硅烃基。

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