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11. 发明申请

US20100056737A1 Process for manufacturing high to ultra high molecular weight polymers using novel bridged metallocene catalysts 有权
标题翻译：使用新型桥连茂金属催化剂制造高分子量超分子量聚合物的方法
公开(公告)号：US20100056737A1
公开(公告)日：2010-03-04
申请号：US12584092
申请日：2009-08-31
申请人： Tim Dickner , Jens Ehlers , Jörg Schottek , Jens Panitzky
发明人： Tim Dickner , Jens Ehlers , Jörg Schottek , Jens Panitzky
IPC分类号： C08F4/42
CPC分类号： C08F10/02 , C08F110/02 , Y10S526/943 , C08F4/61927 , C08F2500/01
摘要： The present invention relates to a process of manufacturing high, very high, and ultra high molecular weight polymers comprising predominantly ethylene monomers. Ethylene is reacted in the presence of a catalyst system to produce a polymer having a viscosimetrically-determined molecular weight of at least 0.7×106 g/mol. The catalyst system generally includes a bridged metallocene catalyst compound, optionally with a co-catalyst. The catalyst is characterized by a zirconium dichloride central functionality and a dimethyl silandiyl bridge between five-membered rings of indenyl groups. Both rings of the metallocene compound are substituted at the 2-position with respect to the dimethyl silandiyl bridge with a C1-C20 carbonaceous group.
摘要翻译：本发明涉及制造主要是乙烯单体的高，非常高和超高分子量聚合物的方法。乙烯在催化剂体系的存在下反应，生成具有至少0.7×106g / mol的粘度测定分子量的聚合物。催化剂体系通常包括桥联茂金属催化剂化合物，任选地具有助催化剂。该催化剂的特征在于二氯化锆中心官能团和五元环茚基之间的二甲基硅烷基桥。相对于具有C1-C20碳质基团的二甲基硅烷基桥，茂金属化合物的两个环在2-位被取代。

12. 发明授权

US07049453B2 “Constrained geometry” metallocenes, method for the production thereof and use of the same for the polymerisation of olefins 有权
标题翻译： “约束几何”金属茂，其制备方法和用于烯烃聚合的方法
公开(公告)号：US07049453B2
公开(公告)日：2006-05-23
申请号：US10508238
申请日：2003-03-24
申请人： Jörg Schottek , Tim Dickner , Jörg Ludwig Schulte
发明人： Jörg Schottek , Tim Dickner , Jörg Ludwig Schulte
IPC分类号： C07F17/00 , B01J31/00 , C08F4/44
CPC分类号： C07F17/02 , C07F17/00 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F10/00 , C08F2410/02 , C08F2420/01 , C08F2420/02 , Y10S526/943 , C08F4/6592 , C08F4/64044 , C08F4/64148
摘要： The present invention relates to a process for preparing specific transition metal compounds, novel transition metal compounds and also catalyst systems and their use for the homo- or copolymerization of olefins.
摘要翻译：本发明涉及一种制备特定过渡金属化合物，新型过渡金属化合物以及催化剂体系的方法及其用于烯烃均聚或共聚合的方法。

13. 发明授权

US07101940B2 Chemical compound, method for the production thereof and its use in catalyst systems for producing polyolefins 有权
标题翻译：化合物，其制备方法及其在制备聚烯烃的催化剂体系中的应用
公开(公告)号：US07101940B2
公开(公告)日：2006-09-05
申请号：US10168719
申请日：2000-12-21
申请人： Jörg Schottek , Heike Gregorius , David Fischer , Iris Kuellmer
发明人： Jörg Schottek , Heike Gregorius , David Fischer , Iris Kuellmer
IPC分类号： C08F4/52 , C08F4/76 , B01J31/14 , C07C211/63 , C07F5/02
CPC分类号： C07F5/062 , C07F5/027 , C08F4/65916 , C08F4/65927 , C08F110/06 , Y10S526/943 , C08F4/65908 , C08F2500/03
摘要： The invention relates to a chemical compound of formula (I), wherein M1 represents an element selected from main groups II, III or IV of the periodic table of elements; x is equal to 1, 2, 3 or 4; y is equal to 2, 3 or 4, and; A represents a cation of main group V of the periodic table of elements; R1 is the same or different and represents a branched or unbranched linear or cyclic C1–C40 group that contains carbon; R2 is the same or different and represents a branched or unbranched linear or cyclic C1–C40 group that contains carbon; R3 represents a branched or unbranched linear or cyclic C1–C40 group that contains carbon, and; R4 represents a hydrogen atom; whereby R2 and R3 are always different from one another
摘要翻译：本发明涉及式（I）的化合物，其中M 1表示选自元素周期表的主要组II，III或IV的元素; x等于1,2,3或4; y等于2,3或4， A表示元素周期表第V族的阳离子; R 1相同或不同，表示含有碳的支链或非支链的直链或环状C 1 -C 40 -C 40基团; R 2相同或不同，表示含碳的支链或非支链的直链或环状C 1 -C 40 -C 40基团; R 3表示含有碳的支链或非支链的直链或环状C 1 -C 40 -C 40基团， R 4表示氢原子; 由此R 2和R 3 3总是彼此不同

14. 发明授权

US06861384B2 Process for preparation of a salt-like chemical compound and its use in catalyst systems for preparing polyolefins 失效
标题翻译：盐类化合物的制备方法及其在制备聚烯烃的催化剂体系中的应用
公开(公告)号：US06861384B2
公开(公告)日：2005-03-01
申请号：US10659163
申请日：2003-09-10
申请人： Jörg Schottek , Gerhard Erker , Gerald Kehr
发明人： Jörg Schottek , Gerhard Erker , Gerald Kehr
IPC分类号： C07F5/02 , C08F4/603 , C08F4/626 , C08F4/6392 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/02 , C08F110/06 , C08F4/64 , C07F5/05
CPC分类号： C08F10/00 , C07F5/027 , C08F4/65912 , C08F4/65916 , C08F4/65922 , C08F110/02 , C08F110/06 , Y10S526/943 , C08F4/61908 , C08F4/65908 , C08F4/603 , C08F2500/15
摘要： A process for preparing salt-like compounds of the formula (1), (C6R115)3MR2 (I) where R1 are identical or different and are each a hydrogen atom, a halogen atom, C1-C20-alkyl, C6-C14-aryl, C1-C10-alkoxy, C2-C10-alkenyl, C7-C20-arylalkyl, C7-C20-alkylaryl, C6-C10-aryloxy, C1-C10-haloalkyl, C6-C10-haloaryl, C2-C10-alkynyl or C3-C20-alkylsilyl, M is an element of main group III of the Periodic Table of the Elements, and R2 is a substituted or unsubstituted heterocycle, and the use of such compounds in catalyst systems for preparing polyolefins.
摘要翻译：制备式（1）的盐类化合物的方法，其中R 1相同或不同，各自为氢原子，卤素原子，C 1 -C 20烷基，C 6 -C 14 - 芳基，C 1 -C 10 - 烷氧基，C 2 -C 10 - 烯基，C 7 -C 20 - 芳烷基，C 7 -C 20烷基芳基，C 6 -C 10 - 芳氧基，C 1 -C 10卤代烷基，C 6 -C 10 - 卤代芳基，C 2 -C 10 - 炔基或C 3 -C 20烷基甲硅烷基， M是元素周期表的主要组III的元素，R 2是取代或未取代的杂环，以及这些化合物在催化剂体系中用于制备聚烯烃的用途。

15. 发明授权

US06600066B1 Method for producing mono-organoboranes or di-organoboranes 失效
标题翻译：制备单有机硼烷或二有机硼烷的方法
公开(公告)号：US06600066B1
公开(公告)日：2003-07-29
申请号：US09868074
申请日：2001-06-14
申请人： Jörg Schottek , Patricia Becker , Iris Küllmer
发明人： Jörg Schottek , Patricia Becker , Iris Küllmer
IPC分类号： C07F502
CPC分类号： C07F5/02 , C07F5/025 , C07F5/066
摘要： A novel process for preparing perhalogenated monoorganoboranes or diorganoboranes which makes it possible to obtain these compounds under conditions which can readily be implemented in the industry is described.
摘要翻译：描述了一种制备全卤代单有机硼烷或二有机硼烷的新方法，其使得可以在可容易地在工业中实施的条件下获得这些化合物成为可能。

16. 发明授权

US06486277B1 Zwitterionic transition metal compound which contains boron 失效
标题翻译：含有硼的两性离子过渡金属化合物
公开(公告)号：US06486277B1
公开(公告)日：2002-11-26
申请号：US09622205
申请日：2000-08-14
申请人： Gerhard Erker , Gerald Kehr , Jörg Schottek , Roland Kratzer
发明人： Gerhard Erker , Gerald Kehr , Jörg Schottek , Roland Kratzer
IPC分类号： C08F464
CPC分类号： C08F10/00 , C07F17/00 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F4/65927 , Y10S526/943 , C08F4/65925
摘要： A boron-containing zwitterionic neutral transition metal compound which can advantageously be used for the polymerization of olefins is described. Here, the use of aluminoxanes, such as methylaluminoxane (MAO), as a cocatalyst can be dispensed with and a high catalyst activity and a good polymer morphology can nevertheless be achieved.
摘要翻译：描述了可有利地用于烯烃聚合的含硼两性离子中性过渡金属化合物。这里，可以省去使用铝氧烷如甲基铝氧烷（MAO）作为助催化剂，并且仍能实现高催化剂活性和良好的聚合物形态。

17. 发明授权

US06458982B1 Transition metal compound, catalyst, its production and its use for the polymerization of olefins 失效
标题翻译：过渡金属化合物，催化剂，其生产及其在烯烃聚合中的应用
公开(公告)号：US06458982B1
公开(公告)日：2002-10-01
申请号：US09515406
申请日：2000-02-29
申请人： Jörg Schottek , Roland Kratzer
发明人： Jörg Schottek , Roland Kratzer
IPC分类号： B01J3100
CPC分类号： C08F10/06 , C08F4/65912 , C08F4/65916 , C08F110/06 , C08F4/65925
摘要： Metallocene catalysts for the preparation of polyolefins, in particular polypropylene having elastomeric properties, having specific heteroaromatics in position 2 or 3 of the indenyl system. Particular preference is given to unbridged metallocene compounds of the formula II: where M, X and R3 to R8 are defined herein.
摘要翻译：用于制备聚烯烃的茂金属催化剂，特别是具有弹性体性质的聚丙烯，在茚基体系的2位或3位具有特异性杂芳族化合物。特别优选式I的未桥连金属茂化合物：其中M，X和R 3至R 8在本文中定义。

18. 发明授权

US07105690B2 Method for producing transition metal compounds and their use for the polymerization of olefins 失效
公开(公告)号：US07105690B2
公开(公告)日：2006-09-12
申请号：US10297054
申请日：2001-05-30
申请人： Jörg Schottek , Gerhard Erker , Klaus Kunz , Steve Döring
发明人： Jörg Schottek , Gerhard Erker , Klaus Kunz , Steve Döring
IPC分类号： C07F9/28 , C07F7/00 , B01J31/00 , C08F4/44
CPC分类号： C07F17/00 , C08F4/65912 , C08F10/00 , C08F110/02 , C08F210/16 , C08F232/00 , Y10S526/943 , C08F4/6592 , C08F210/14
摘要： The invention relates to a method for producing special transition metal compounds, to novel transition metal compounds and to their use for the polymerization of olefins.

19. 发明授权

US07034173B2 Chemical products suited for use as co-catalysts, method for the preparation thereof and their use in catalyst systems for producing polyolefins 有权
公开(公告)号：US07034173B2
公开(公告)日：2006-04-25
申请号：US10276782
申请日：2001-05-19
申请人： Jörg Schottek
发明人： Jörg Schottek
IPC分类号： C07F5/00 , C07F5/06
CPC分类号： C07F5/066 , C07F5/062
摘要： The invention relates to chemical products which are suited for use as co-catalysts and which can be obtained by reacting a compound of formula (I), M1R1R2(R3)m with a compound of formula (II), (R4X)q-(G)*(M2R5R6)g. In formula (I), R1, R2 and R3 are the same or different and represent a hydrogen atom, C1–C20 alkyl, C1–C20 alkyl halide, C6–C20 aryl, C6–C20 aryl halide, C7–C40 arylalkyl, C7–C40 arylalkyl halide, C7–C40 alkylaryl or C7–C40 alkylaryl halide; M1 represents an element of the second or third main group of the periodic table of elements, and; m equals 0 or 1, whereby m is equal to 1 when M1 represents an element of the third main group, and m is equal to 0 when M1 represents an element of the second main group. In formula (II), substituents R4X, which contain hetero atoms, is located on a base body G, and: groups R4 are the same or different and represent hydrogen, C1–C20 alkyl, C1–C20 alkyl halide, C6–C20 aryl, C6–C20 aryl halide, C7–C40 arylalkyl, C7–C40 arylalkyl halide, C7–C40 akylaryl or C7–C40 alkylaryl halide; X represents an element of the fourth, fifth or sixth main group of the periodic table of elements; G represents at least bivalent C1–C20 alkylene, C1–C20 alkylene halide, C1–C10 alkylenoxy, C6–C40 arylene, C6–C40 arylene halide, C6–C40 arylenoxy, C7–C40 arylalkylene, C7–C40 arylalkylene halide, C7–C40 alkylarylene, C7–C40 alkylarylene halide; M2 represents an element of the fourth, fifth or sixth main group of the periodic table of elements; R5 and R6, independent of one another, are the same or different and represent a hydrogen atom, C1–C20 alkyl, C1–C10 alkoxy, C2–C10 alkenyl, C7–C20 arylalkyl, C7–C20 alkylaryl, C6–C10 aryloxy, C1–C10 alkyl halide; q is a whole number ranging from 2 to 100, and; g is a whole number ranging from 1 to 100. The invention also relates to a method for preparing the inventive chemical products, and to their use in catalyst systems for producing polyolefins.

20. 发明授权

US06953829B2 Catalyst system and the use thereof 失效
标题翻译：催化剂体系及其用途
公开(公告)号：US06953829B2
公开(公告)日：2005-10-11
申请号：US10168646
申请日：2000-12-13
申请人： Roland Kratzer , Cornelia Fritze , Jörg Schottek
发明人： Roland Kratzer , Cornelia Fritze , Jörg Schottek
IPC分类号： C08F4/649 , B01J31/02 , B01J31/14 , B01J31/16 , B01J31/22 , C08F4/64 , C08F4/646 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F4/622 , C08F4/642
CPC分类号： B01J31/1608 , B01J31/0237 , B01J31/14 , B01J31/1616 , B01J31/2295 , B01J2531/46 , B01J2531/48 , B01J2531/49 , C08F4/65908 , C08F4/65912 , C08F4/65927 , C08F10/00 , C08F4/65916
摘要： A catalyst system comprising at least one metallocene, at least one cocatalyst, at least one support material and, if desired, further organometallic compounds is described.The catalyst system can advantageously be used for the polymerization of olefins and displays a high catalyst activity and gives a good polymer morphology without it being necessary to use aluminoxanes such as methylaluminoxane (MAO), which usually has to be used in high excess, as cocatalyst.
摘要翻译：描述了包含至少一种茂金属，至少一种助催化剂，至少一种载体材料和如果需要的其它有机金属化合物的催化剂体系。催化剂体系可以有利地用于烯烃的聚合并显示出高的催化剂活性，并产生良好的聚合物形态，而不需要使用铝氧烷如甲基铝氧烷（MAO）（通常必须以高过量使用）作为助催化剂。

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