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11. 发明授权

US5098953A Method for producing thermoplastic resin compositions 失效
标题翻译：生产热塑性树脂组合物的方法
公开(公告)号：US5098953A
公开(公告)日：1992-03-24
申请号：US647200
申请日：1991-01-28
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
IPC分类号： C08G59/00 , C08G59/20 , C08G59/32 , C08G59/40 , C08K5/00 , C08K5/05 , C08K5/053 , C08K5/09 , C08K5/092 , C08K5/1515 , C08K5/17 , C08K5/353 , C08L63/00 , C08L67/00 , C08L67/02
CPC分类号： C08K5/0025 , C08L67/02
摘要： Disclosed is a method for producing a thermoplastic resin composition which can be easily molded into articles having good balance in properties and good appearance. Said method comprises melt-kneading (A) 60-97 parts by weight of a saturated polyester resin and (B) 40-3 parts by weight of an epoxy group-containing ethylene copolymer and then melt-kneading the resulting composition with (C) 0.01-20 parts by weight of a polyfunctional compound containing in one molecule at least two functional groups having reactivity with epoxy group, carboxyl group or hydroxyl group to carry out partial crosslinking reaction.

12. 发明授权

US5086116A Method for producing thermoplastic resin composition 失效
公开(公告)号：US5086116A
公开(公告)日：1992-02-04
申请号：US513940
申请日：1990-04-24
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
IPC分类号： C08G59/00 , C08G59/20 , C08G59/32 , C08G59/40 , C08K5/00 , C08K5/05 , C08K5/053 , C08K5/09 , C08K5/092 , C08K5/1515 , C08K5/17 , C08K5/353 , C08L63/00 , C08L67/00 , C08L67/02
CPC分类号： C08K5/0025 , C08L67/02
摘要： Disclosed is a method for producing a thermoplastic resin composition which can be easily molded into articles having good balance in properties and good appearance. Said method comprises melt-kneading (A) 60-97 parts by weight of a saturated polyester resin and (B) 40-3 parts by weight of an epoxy group-containing ethylene copolymer and then melt-kneading the resulting composition with (C) 0.01-20 parts by weight of a polyfunctional compound containing in one molecule at least two functional groups having reactivity with epoxy group, carboxyl group or hydroxyl group to carry out partial crosslinking reaction.

13. 发明授权

US5047479A Thermoplastic resin composition 失效
标题翻译：热塑性树脂组合物
公开(公告)号：US5047479A
公开(公告)日：1991-09-10
申请号：US396786
申请日：1989-08-21
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Jinsho Nambu
IPC分类号： C08K5/00 , C08K5/09 , C08K5/17 , C08K5/21 , C08K5/24 , C08K5/3492 , C08K5/353 , C08L77/00
CPC分类号： C08L77/00
摘要： A thermoplastic resin composition is disclosed, which is obtained by melt-kneading (A) from 60 to 97 parts by weight of a polyamide resin and (B) from 3 to 40 parts by weight of an ethylene copolymer comprising (a) from 40 to 90% by weight of an ethylene unit, (b) from 5 to 60% by weight of an alkyl .alpha., .beta.-unsaturated carboxylate unit, and (c) from 0.3 to 10% by weight of a maleic anhydride unit and then melt-kneading the resulting composition with (C) from 0.01 to 20 parts by weight of a polyfunctional compound having at least two functional groups having reactivity to a carboxyl group, a carboxylic acid anhydride group or an amino group per molecule to effect partial crosslinking reaction. The composition provides molded articles having a good balance of physical properties and satisfactory appearance.

14. 发明授权

US5155159A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US5155159A
公开(公告)日：1992-10-13
申请号：US672985
申请日：1991-03-21
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi
IPC分类号： C08K3/20 , C08K3/22 , C08K5/17 , C08K5/21 , C08L23/08 , C08L77/00
CPC分类号： C08L77/00 , C08L23/0853 , C08L23/0869
摘要： A thermoplastic elastomer composition having a flexural modulus as defined in JIS K7203-1982 of from 500 to 15,000 kg/cm.sup.2, which is obtainable by melt kneading(A) from 20 to 60 parts by weight of a polyamide resin with(B) from 40 to 80 parts by weight of an ethylene copolymer comprising (a) from 40 to 90% by weight of an ethylene unit, (b) from 5 to 60% by weight of an .alpha.,.beta.-unsaturated carboxylic acid alkyl ester unit, and (c) from 0.3 to 10% by weight of a maleic anhydride unit, to obtain a composition (I), and further melt kneading 100 parts by weight of the composition (I) with(C) from 0.01 to 10 parts by weight of magnesium hydroxide having a specific surface area of no more than 20 m.sup.2 /g as measured by the Brunauer-Emmett-Teller method, is disclosed.
摘要翻译：通过熔融捏合（A）20〜60重量份的聚酰胺树脂（B）为40〜40重量份，得到JIS K7203-1982中规定的弯曲弹性模量为500〜15000kg / cm 2的热塑性弹性体组合物至80重量份的乙烯共聚物，其包含（a）40至90重量％的乙烯单元，（b）5至60重量％的α，β-不饱和羧酸烷基酯单元和（ c）0.3〜10重量％的马来酸酐单元，得到组合物（I），进一步将100重量份组合物（I）与（C）熔融捏合0.01〜10重量份的镁公开了通过Brunauer-Emmett-Teller方法测量的比表面积不大于20m 2 / g的氢氧化物。

15. 发明授权

US5405909A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US5405909A
公开(公告)日：1995-04-11
申请号：US147466
申请日：1993-10-26
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi , Kenzo Chikanari
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi , Kenzo Chikanari
IPC分类号： C08K5/00 , C08G59/00 , C08G81/00 , C08K5/053 , C08K5/092 , C08K5/17 , C08K5/21 , C08K5/405 , C08L23/08 , C08L37/00 , C08L53/00 , C08L63/00 , C08L67/00 , C08L67/02 , C08L71/00
CPC分类号： C08L23/0884 , C08L63/00 , C08L67/02 , C08K5/053 , C08K5/092 , C08K5/17 , C08K5/21 , C08K5/405 , C08L2205/02 , C08L2205/03 , C08L2205/035 , C08L23/0869 , C08L2310/00 , C08L53/00
摘要： A thermoplastic elastomer composition which is useful for bumper, boot, sound absorbing gear, sports shoes etc. is provided by mixing the following (A)-(D).A: 30-58 parts by wt of saturated polyester resin,B: 42-70 parts by wt of an epoxy group-containing ethylene copolymer ofa) 50-99% by wt of ethylene unit,b) 0.1-30% by wt of unsaturated carboxylic acid glycidyl ester unit or unsaturated glycidyl ether unit andc) 0-49% by wt of ethylenically unsaturated ester unitC: 0.01-20 parts by wt of specific polyfunctional compound containing two or more functional groups, andD: 1-30 parts by wt of block copolyether ester elastomer.The amounts of C and D are based on 100 parts of A and B.
摘要翻译：通过混合以下（A） - （D）来提供用于保险杠，靴子，吸音齿轮，运动鞋等的热塑性弹性体组合物。 A：30-58重量份的饱和聚酯树脂，B：42-70重量份的a）50-99重量％的乙烯单元的含环氧基的乙烯共聚物，b）0.1-30重量％的不饱和羧酸缩水甘油酯单元或不饱和缩水甘油醚单元，和c）0-49重量％的烯键式不饱和酯单元C：0.01-20重量份含有两个或更多个官能团的特定多官能化合物，D：1- 30重量份嵌段共聚醚酯弹性体。 C和D的量基于A和B的100份。

16. 发明授权

US6017999A Method for producing impact-resistant polyester resin compositions 失效
标题翻译：耐冲击聚酯树脂组合物的制造方法
公开(公告)号：US6017999A
公开(公告)日：2000-01-25
申请号：US312621
申请日：1994-09-27
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi , Kenzo Chikanari
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Kentaro Mashita , Noboru Yamaguchi , Kenzo Chikanari
IPC分类号： C08J5/00 , C08G59/00 , C08G81/00 , C08K5/00 , C08L23/08 , C08L37/00 , C08L53/00 , C08L63/00 , C08L67/00 , C08L67/02 , C08L71/00 , C08L33/14
CPC分类号： C08L23/08 , C08L63/00 , C08L67/02 , C08L2205/08 , C08L23/0884 , C08L53/00
摘要： A saturated polyester resin composition excellent in impact resistance is prepared by melt kneading (A) 30-58 parts by weight of a saturated polyester resin, (B) 42-70 parts by weight of an epoxy group-containing ethylene copolymer comprising (a) 50-99% by weight of ethylene unit, (b) 0.1-30% by weight of unsaturated carboxylic acid glycidyl ester unit or unsaturated glycidyl ether unit, and (c) 0-49% by weight of ethylenically unsaturated ester compound unit, (C) 0.01-20 parts by weight of a polyfunctional compound containing at least two specific functional groups of amino groups, carboxyl groups, carboxylic acid anhydride groups, hydroxyl groups or ##STR1## unit (wherein X and Y are both oxygen atoms or sulfur atoms or one of them is an oxygen atom and another is a sulfur atom) and (D) 0-30 parts by weight of a block copolyether ester elastomer, the amounts of (C) and (D) being based on 100 parts by weight of (A) plus (B), thereby to obtain a former-stage composition (I) and furthermore melt kneading the resulting composition (I) with (E) 50-1000 parts by weight of a saturated polyester resin and (F) 0-30 parts by weight of a block copolyether ester elastomer at a later-stage.
摘要翻译：通过熔融捏合（A）30-58重量份的饱和聚酯树脂，（B）42-70重量份的包含（a）的含环氧基的乙烯共聚物来制备耐冲击性优异的饱和聚酯树脂组合物， 50-99重量％的乙烯单元，（b）0.1-30重量％的不饱和羧酸缩水甘油酯单元或不饱和缩水甘油醚单元，和（c）0-49重量％的烯属不饱和酯化合物单元，（ C）0.01-20重量份含有氨基，羧基，羧酸酐基团，羟基或单元的至少两个特定官能团的多官能化合物（其中X和Y都是氧原子或硫原子或其中之一它们是氧原子，另一个是硫原子）和（D）0-30重量份的嵌段共聚醚酯弹性体，（C）和（D）的量基于100重量份的（A）加（B），从而得到前期组合物（I），进而熔融将得到的组合物（I）与（E）50-1000重量份的饱和聚酯树脂和（F）0-30重量份的嵌段共聚醚酯弹性体在后期捏合。

17. 发明授权

US5367013A Process for producing reinforced crystalline engineering plastic composition 失效
标题翻译：生产强化结晶工程塑料成分的方法
公开(公告)号：US5367013A
公开(公告)日：1994-11-22
申请号：US958727
申请日：1992-10-09
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Noboru Yamaguchi , Kenzo Chikanari
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Noboru Yamaguchi , Kenzo Chikanari
IPC分类号： C08L23/08 , C08L67/02 , C08L77/00 , C08L81/02 , C08L101/00 , C08K3/00
CPC分类号： C08L81/02 , C08L101/00 , C08L67/02 , C08L77/00 , C08L2205/06 , C08L23/08
摘要： A process for producing a reinforced crystalline engineering plastic composition is disclosed, comprising melt-kneading (A) from 60 to 97 parts by weight of a crystalline engineering plastic and (B) from 5 to 100 parts by weight, per 100 parts by weight of the sum of (A) and (C), of glass fibers and melt-kneading the resulting mixture with (C) from 3 to 40 parts by weight of an epoxy- or acid anhydride-containing ethylene copolymer. The composition obtained provides, with excellent moldability, a molded article having an improved appearance while exhibiting well-balanced mechanical and thermal properties.
摘要翻译：公开了一种生产增强结晶工程塑料组合物的方法，包括将（A）60至97重量份的结晶工程塑料和（B）5至100重量份熔体捏合（A），相对于每100重量份（A）和（C）的总和，并将得到的混合物与（C）熔融捏合3至40重量份的含环氧或含酸酐的乙烯共聚物。获得的组合物具有优异的成型性，其具有改进外观的模制品，同时具有良好平衡的机械和热性能。

18. 发明授权

US5296552A Adhesive resin composition 失效
标题翻译：粘合剂树脂组合物
公开(公告)号：US5296552A
公开(公告)日：1994-03-22
申请号：US840805
申请日：1992-02-25
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Mitsuyuki Okada , Harunori Fujita
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Mitsuyuki Okada , Harunori Fujita
IPC分类号： C08F8/00 , B29B7/46 , C08F255/00 , C08J3/00 , C08L23/26 , C09J151/00 , C09J151/06
CPC分类号： C09J151/06 , B29C47/366 , C08F255/00
摘要： An adhesive resin composition is obtained by mixing at least one member (C) selected from the group consisting of unsaturated carboxylic acids and the derivatives thereof, a free-radical initiator (D), and a mixture consisting of a crystalline polyolefin resin (A) and an amorphous or low crystalline olefin copolymer of ethylene and an .alpha.-olefin (B), to obtain a precursor mixture, melt-kneading the precursor mixture in the first half of an extruder having at least one side feeder, to obtain a modified precursor mixture, and feeding a crystalline polyolefin resin (E) from the side feeder of the extruder and mixing the resin (E) with the modified precursor mixture.The adhesive resin composition has good extrudability and exhibits high adhesive property to polar materials such as polar polymeric materials and the like.
摘要翻译：通过混合至少一种选自不饱和羧酸及其衍生物的组分（C），自由基引发剂（D）和由结晶聚烯烃树脂（A）组成的混合物，得到粘合剂树脂组合物，和乙烯与（α） - 烯烃（B）的无定形或低结晶烯烃共聚物，以获得前体混合物，在具有至少一个侧进料器的挤出机的前半部分中熔融捏合前体混合物，得到并且从挤出机的侧进料器进料结晶聚烯烃树脂（E）并将树脂（E）与改性前体混合物混合。粘合性树脂组合物具有良好的挤出性，并且对极性材料如极性聚合物材料等显示出高粘合性。

19. 发明授权

US5290865A Process for producing a lactam compound graft copolymer of ethylene copolymer 失效
标题翻译：制备乙烯共聚物的内酰胺化合物接枝共聚物的方法
公开(公告)号：US5290865A
公开(公告)日：1994-03-01
申请号：US984236
申请日：1992-12-01
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Toshio Kawakita
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Toshio Kawakita
IPC分类号： C08F8/30 , C08L77/00
CPC分类号： C08F8/30
摘要： A process for producing a graft copolymer comprising melt-blending:(A) 1 to 90 parts by weight of an ethylene copolymer, based on the weight of the graft copolymer, comprising (a) 40 to 99.9% by weight of ethylene units, (b) 0 to 60% by weight of .alpha.,.beta.-unsaturated carboxylic acid alkyl ester units, and (c) 0.1 to 10% by weight of maleic anhydride units;(B) 0.1 to 10 moles of a lactam metal salt compound per mole of the maleic anhydride units (c) of the ethylene copolymer (A); and(C) 10 to 99 parts by weight of a lactam compound, based on the weight of the graft copolymer,which results in a graft copolymer having high impact strength, high flexibility, satisfactory dyeability, and well-balanced physical properties over a wide temperature range.
摘要翻译：一种制备接枝共聚物的方法，包括熔融共混：（A）1-90重量份乙烯共聚物，基于接枝共聚物的重量，包括（a）40-99.9重量％的乙烯单元，（ b）0至60重量％的（α），（β-）不饱和羧酸烷基酯单元，和（c）0.1至10重量％的马来酸酐单元; （B）每摩尔乙烯共聚物（A）的马来酸酐单元（c）为0.1〜10摩尔的内酰胺金属盐化合物; 和（C）10至99重量份的内酰胺化合物，基于接枝共聚物的重量，其导致接枝共聚物具有高冲击强度，高柔性，令人满意的可染性和在宽的物理性能上的良好平衡温度范围。

20. 发明授权

US5180784A Adhesive resin composition 失效
标题翻译：粘合树脂组合物
公开(公告)号：US5180784A
公开(公告)日：1993-01-19
申请号：US869179
申请日：1992-04-16
申请人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Mitsuyuki Okada , Harunori Fujita
发明人： Tadayuki Ohmae , Yoshiki Toyoshima , Hisao Tanaka , Mitsuyuki Okada , Harunori Fujita
IPC分类号： C08L23/06 , C08L23/00 , C08L23/08 , C08L23/16 , C09J123/04 , C09J123/08
CPC分类号： C09J123/04 , C09J123/08 , Y10T428/31649 , Y10T428/31757 , Y10T428/31797 , Y10T428/31913
摘要： An adhesive resin composition is disclosed, comprising:(A) from 2 to 98% by weight of an ethylene copolymer comprising from 50 to 90% by weight of ethylene, from 0 to 49% by weight of an .alpha.,.beta.-unsaturated carboxylic acid alkyl ester, and from 0.5 to 10% by weight of maleic anhydride, with the sum of these monomers being 100% by weight;(B) from 2 to 98% by weight of a crystalline polyethylene resin comprising either an ethylene homopolymer or a copolymer of ethylene and an .alpha.-olefin having 3 or more carbon atoms, with an ethylene content being 90% by weight or more; and(C) from 2 to 50% by weight of a non-crystalline or low crystalline olefin copolymer rubber comprising a copolymer of ethylene and an .alpha.-olefin having 3 or more carbon atoms, with the sum of the components (A), (B) and (C) being 100% by weight.

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