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11. 发明授权

US06150291A Method of abating NO.sub.x and preparation of catalytic material therefor 失效
标题翻译：降低NOx的方法及其催化剂的制备
公开(公告)号：US06150291A
公开(公告)日：2000-11-21
申请号：US250652
申请日：1999-02-16
申请人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
发明人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
IPC分类号： B01D53/86 , B01D53/94 , B01J29/40 , B01J29/44 , B01J29/70 , B01J29/04
CPC分类号： B01J29/44 , B01D53/9418 , B01D2251/208 , B01D2255/1021 , B01D2255/1026 , B01D2255/502 , B01D2255/504 , B01D2255/912 , Y02C20/10
摘要： A method for reducing gaseous nitrogen oxides present in a gas stream by reaction with a reductant species is practiced by flowing the gas stream under lean NO.sub.X -reducing conditions in contact with a catalytic material containing a catalytically effective amount of a catalytic species, e.g., a platinum group metal, and a reductant storage material, e.g., a zeolite, effective for storing reductant species for reaction with NO.sub.X, and providing an intermittent supply of the reductant to the gas stream. The catalytic material may be prepared in any manner, but one method is to incorporate a catalytically effective amount of the platinum into a template-bearing molecular sieve material, preferably ZSM-5, to hinder the platinum from being incorporated into the pores of the molecular sieve material, and then calcining the molecular sieve material, whereby the template is removed from the molecular sieve material after the platinum is incorporated therein. Another method is to add a blocking agent to the molecular sieve material, then incorporate the platinum therein, and then calcine the material to remove the blocking agent. The catalytic material may contain less than about two percent by weight of zeolite plus platinum, e.g., less than about 0.5%, or from about 0.025% to 0.1% or 0.2% platinum.
摘要翻译：通过与还原剂物质反应来还原存在于气流中的气态氮氧化物的方法是通过在贫NOX还原条件下与含有催化有效量的催化物质（例如，铂族金属和还原剂储存材料，例如有效地存储用于与NOX反应的还原剂物质的沸石，以及向气流中间歇地供应还原剂。催化材料可以以任何方式制备，但是一种方法是将催化有效量的铂掺入含模板的分子筛材料，优选ZSM-5中，以阻止铂结合到分子的孔中筛分材料，然后煅烧分子筛材料，由此在引入铂后，从分子筛材料中除去模板。另一种方法是向分子筛材料中加入封闭剂，然后在其中加入铂，然后煅烧该材料以除去封闭剂。催化材料可以含有小于约2重量％的沸石加铂，例如小于约0.5％，或约0.025％至0.1％或0.2％的铂。

12. 发明授权

US5792436A Method for using a regenerable catalyzed trap 失效
标题翻译：使用可再生催化陷阱的方法
公开(公告)号：US5792436A
公开(公告)日：1998-08-11
申请号：US645301
申请日：1996-05-13
申请人： Jennifer S. Feeley , Robert J. Farrauto , Michel Deeba , Jordan K. Lampert
发明人： Jennifer S. Feeley , Robert J. Farrauto , Michel Deeba , Jordan K. Lampert
IPC分类号： B01D53/86 , B01D53/94 , B01J23/42 , B01J23/63 , B01J23/656 , F01N3/08 , F01N3/10 , F01N3/20 , B01D53/56 , B01D53/75
CPC分类号： F01N3/085 , B01D53/8609 , B01D53/8671 , B01D53/9431 , F01N3/0814 , F01N3/0871 , B01D2257/00 , B01D2257/302 , F01N2250/12 , F01N2330/06 , F01N2570/14 , F01N2610/03
摘要： A method of at least periodically removing from a lean gaseous stream a sorbable component such as SO.sub.x includes passing the gaseous stream through a trap member having an oxidation catalyst combined with a sorbent material at a temperature within the sorbing temperature range of the sorbent material. The sorbed component is periodically removed by introducing a combustible component into the gaseous stream and oxidizing it on the trap member to thermally desorb the sorbed component. The amount of combustible component introduced is limited to maintain the gaseous stream composition lean, but is sufficient to increase the surface temperature of at least part of the trap member to above the bulk temperature of the gaseous stream. Sorbing and desorbing periods are alternated and a composition and an apparatus to carry out the process is provided.
摘要翻译：至少周期性地从贫气流中除去可吸收组分如SOx的方法包括使气流通过具有与吸附剂材料组合的氧化催化剂的捕集构件，所述氧化催化剂在吸附剂材料的吸附温度范围内。通过将可燃组分引入气流中并在捕集构件上氧化吸附组分以热解吸附吸附的组分来定期除去吸附的组分。引入的可燃组分的量被限制以保持气流组合物变稀，但足以使至少部分捕集构件的表面温度升至高于气流体积的温度。曳引和解吸时间是交替的，并且提供了一个组合物和一个执行该过程的装置。

13. 发明授权

US6080377A Method of abating NO.sub.x and a catalytic material therefor 失效
标题翻译：减轻NOx及其催化材料的方法
公开(公告)号：US6080377A
公开(公告)日：2000-06-27
申请号：US430065
申请日：1995-04-27
申请人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
发明人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
IPC分类号： B01D53/86 , B01D53/94 , B01J29/40 , B01J29/44 , B01J29/70 , B01J8/00
CPC分类号： B01J29/44 , B01D53/9418 , B01D2251/208 , B01D2255/1021 , B01D2255/1026 , B01D2255/502 , B01D2255/504 , B01D2255/912 , Y02C20/10
摘要： A method for reducing gaseous nitrogen oxides present in a gas stream by reaction with a reductant species is practiced by flowing the gas stream under lean NO.sub.X -reducing conditions in contact with a catalytic material containing a catalytically effective amount of a catalytic species, e.g., a platinum group metal, and a reductant storage material, e.g., a zeolite, effective for storing reductant species for reaction with NO.sub.X, and providing an intermittent supply of the reductant to the gas stream. The catalytic material may be prepared in any manner, but one method is to incorporate a catalytically effective amount of the platinum into a template-bearing molecular sieve material, preferably ZSM-5 zeolite, to hinder the platinum from being incorporated into the pores of the molecular sieve material, and then calcining the molecular sieve material, whereby the template is removed from the molecular sieve material after the platinum is incorporated therein. Another method is to add a blocking agent to the molecular sieve material, then incorporate the platinum therein, and then calcine the material to remove the blocking agent. The catalytic material may contain less than about two percent by weight of zeolite plus platinum, e.g., less than about 0.5%, or from about 0.025% to 0.1% or 0.2% platinum.
摘要翻译：通过与还原剂物质反应来还原存在于气流中的气态氮氧化物的方法是通过在贫NOX还原条件下与含有催化有效量的催化物质（例如，铂族金属和还原剂储存材料，例如有效地存储用于与NOX反应的还原剂物质的沸石，以及向气流中间歇地供应还原剂。催化材料可以以任何方式制备，但是一种方法是将催化有效量的铂掺入含模板的分子筛材料，优选ZSM-5沸石中，以阻止铂被引入到分子筛材料，然后煅烧分子筛材料，由此在引入铂后，从分子筛材料中除去模板。另一种方法是向分子筛材料中加入封闭剂，然后在其中加入铂，然后煅烧该材料以除去封闭剂。催化材料可以含有小于约2重量％的沸石加铂，例如小于约0.5％，或约0.025％至0.1％或0.2％的铂。

14. 发明授权

US07759533B2 Lightly branched higher olefin oligomerization with surface modified zeolite catalyst 有权
标题翻译：用表面改性沸石催化剂轻支化高级烯烃低聚
公开(公告)号：US07759533B2
公开(公告)日：2010-07-20
申请号：US11973101
申请日：2007-10-05
申请人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
发明人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
IPC分类号： C07C2/12
CPC分类号： C07C2/12 , B01J29/7076 , B01J29/7092 , B01J29/7096 , B01J2229/123 , B01J2229/18 , B01J2229/20 , B01J2229/42
摘要： A substantially surface-deactivated catalyst composition that is stable at least to 300° C. The catalyst includes a zeolite catalyst (e.g., ZSM-22, ZSM-23, or ZSM-57) having active internal Brönsted acid sites and a surface-deactivating amount of a rare earth or yttrium oxide (e.g., chosen from lanthanum oxide or lanthanides oxide). This catalyst is preferably used in a process for producing a higher olefin by oligomerizing a light olefin, wherein the process includes contacting a light olefin under oligomerization conditions with the substantially surface-deactivated catalyst composition.
摘要翻译：基本上表面失活的催化剂组合物，其稳定至少为300℃。催化剂包括具有活性内部布朗斯台德酸位点和表面失活的沸石催化剂（例如，ZSM-22，ZSM-23或ZSM-57）稀土或氧化钇的量（例如，选自氧化镧或氧化镧）。该催化剂优选用于通过低聚烯烃生产高级烯烃的方法，其中该方法包括在低聚条件下使轻质烯烃与基本上表面失活的催化剂组合物接触。

15. 发明申请

US20080175765A1 High throughput, microwave energy heated continuous hydrothermal synthesis apparatus 审中-公开
标题翻译：高通量，微波能量加热连续水热合成装置
公开(公告)号：US20080175765A1
公开(公告)日：2008-07-24
申请号：US12001907
申请日：2007-12-13
申请人： Guang Cao , Sabato Miseo , Stu L. Soled , Jennifer S. Feeley
发明人： Guang Cao , Sabato Miseo , Stu L. Soled , Jennifer S. Feeley
IPC分类号： B01J19/12
CPC分类号： B01J37/10 , B01J23/8885 , B01J37/0036
摘要： The present invention is a high throughput apparatus. The apparatus is an automated multi-channel preparation module that prepares a synthesis mixture, microwave heating zone, product collection vessels, and a means for continuously transferring the synthesis mixture through the apparatus.
摘要翻译：本发明是高产量装置。该装置是一种自动多通道制备模块，其制备合成混合物，微波加热区，产物收集容器以及用于将合成混合物连续转移通过该装置的装置。

16. 发明授权

US06726850B1 Catalytic partial oxidation using staged oxygen addition 失效
标题翻译：使用分期加氧的催化部分氧化
公开(公告)号：US06726850B1
公开(公告)日：2004-04-27
申请号：US09484378
申请日：2000-01-14
申请人： Sebastian C. Reyes , Jennifer S. Feeley , Frank Hershkowitz , Harry W. Deckman , Ioannis P. Androulakis
发明人： Sebastian C. Reyes , Jennifer S. Feeley , Frank Hershkowitz , Harry W. Deckman , Ioannis P. Androulakis
IPC分类号： C01B326
CPC分类号： C01B3/386 , C01B2203/0261 , C01B2203/061 , C01B2203/062 , C01B2203/065 , C01B2203/1011 , C01B2203/1029 , C01B2203/1052 , C01B2203/1064 , C01B2203/1082 , C01B2203/1241 , C01B2203/1276
摘要： A multistage catalytic partial oxidation (CPO) process for oxidizing a hydrocarbon feedstream comprising C1-C4 hydrocarbons, with an oxygen-containing feedstream to produce a product comprising CO and H2, also known as synthesis gas or syngas. The process employs a CPO catalyst, and controlled process features, including: (A) the total oxygen requirement for the process is introduced incrementally, in more than one reaction stage, using an oxygen-containing feedstream at more than one feed point in the process, each stage including a catalyst; (B) the oxygen-containing feedstream, hydrocarbon feedstream and, in reaction stages after the first of said multiple stages, the intermediate product produced in the prior stage, are mixed for a period of time, after they are brought into contact with one another, of less than about 1 millisecond to form a substantially uniform mixture, wherein the mixture is then contacted with the catalyst; (C) the oxygen-containing feedstream and the hydrocarbon feedstream are preheated prior to entry into the first stage, to a temperature of from about 450° C. to less than about 1,000° C.; and (D) the mixture temperature of the product in each stage following the first stage is from greater than about 600° C. to less than about 1,000° C. Preferably, the process comprises less than or equal to about five stages, the first stage preheat temperature recited in step (C) is greater than about 550° C. and the mixture temperature of the product in each stage following the first stage is at least 700° C.
摘要翻译：用于将包含C1-C4烃的烃进料流与含氧进料流氧化以产生包含CO和H 2的产物（也称为合成气或合成气）的多级催化部分氧化（CPO）方法。该方法采用CPO催化剂和受控工艺特征，包括：（A）在多于一个反应阶段中，使用含氧进料流在多于一个进料点的过程中逐步引入该方法的总氧需求量，每个阶段包括催化剂; （B）含氧进料流，烃类原料流，在上述多阶段第一阶段后的反应阶段中，将前一阶段生产的中间产物在彼此接触后混合一段时间，小于约1毫秒以形成基本均匀的混合物，其中混合物然后与催化剂接触; （C）在进入第一阶段之前将含氧进料流和烃进料流预热至约450℃至小于约1,000℃的温度; 和（D）在第一阶段之后的每个阶段中的产物的混合物温度为大于约600℃至小于约1000℃。优选地，该方法包括小于或等于约五个阶段，第一阶段步骤（C）中所述的阶段预热温度大于约550℃，并且在第一阶段之后的每个阶段中的产品的混合物温度为至少700℃

17. 发明授权

US06455597B2 Catalytic partial oxidation — particulate catalysts 失效
标题翻译：催化部分氧化 - 颗粒催化剂
公开(公告)号：US06455597B2
公开(公告)日：2002-09-24
申请号：US09791985
申请日：2001-02-23
申请人： Keith L. Hohn , Lanny D. Schmidt , Sebastian C. Reyes , Jennifer S. Feeley
发明人： Keith L. Hohn , Lanny D. Schmidt , Sebastian C. Reyes , Jennifer S. Feeley
IPC分类号： C07C2700
CPC分类号： C01B3/386 , C01B3/40 , C01B2203/0261 , C01B2203/062 , C01B2203/1017 , C01B2203/1023 , C01B2203/1047 , C01B2203/1052 , C01B2203/1064 , C01B2203/1082 , C01B2203/1241 , Y02P20/52
摘要： Catalytic partial oxidation is effected in the presence of a supported, Group VIII metal catalyst by reacting a light hydrocarbon with an oxygen containing gas, the catalyst support being in a preferred size range.
摘要翻译：在负载的VIII族金属催化剂的存在下，通过使轻质烃与含氧气体反应，催化剂载体处于优选的尺寸范围内进行催化部分氧化。

18. 发明申请

US20100248944A1 Lightly Branched Higher Olefin Oligomerization with Surface Modified Zeolite Catalyst 审中-公开
标题翻译：用表面改性沸石催化剂轻分支高级烯烃低聚
公开(公告)号：US20100248944A1
公开(公告)日：2010-09-30
申请号：US12796269
申请日：2010-06-08
申请人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
发明人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
IPC分类号： B01J29/40
CPC分类号： C07C2/12 , B01J29/7076 , B01J29/7092 , B01J29/7096 , B01J2229/123 , B01J2229/18 , B01J2229/20 , B01J2229/42
摘要： A substantially surface-deactivated catalyst composition that is stable at least to 300° C. The catalyst includes a zeolite catalyst (e.g., ZSM-22, ZSM-23, or ZSM-57) having active internal Brönsted acid sites and a surface-deactivating amount of a rare earth or yttrium oxide (e.g., chosen from lanthanum oxide or lanthanides oxide). This to catalyst is preferably used in a process for producing a higher olefin by oligomerizing a light olefin, wherein the process includes contacting a light olefin under oligomerization conditions with the substantially surface-deactivated catalyst composition.
摘要翻译：基本上表面失活的催化剂组合物，其稳定至少为300℃。催化剂包括具有活性内部布朗斯台德酸位点和表面失活的沸石催化剂（例如，ZSM-22，ZSM-23或ZSM-57）稀土或氧化钇的量（例如，选自氧化镧或氧化镧）。该催化剂优选用于通过低聚烯烃生产高级烯烃的方法，其中该方法包括在低聚条件下使轻质烯烃与基本上表面失活的催化剂组合物接触。

19. 发明申请

US20090093663A1 Lightly branched higher olefin oligomerization with surface modified zeolite catalyst 有权
标题翻译：用表面改性沸石催化剂轻支化高级烯烃低聚
公开(公告)号：US20090093663A1
公开(公告)日：2009-04-09
申请号：US11973101
申请日：2007-10-05
申请人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
发明人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
IPC分类号： C07C2/12
CPC分类号： C07C2/12 , B01J29/7076 , B01J29/7092 , B01J29/7096 , B01J2229/123 , B01J2229/18 , B01J2229/20 , B01J2229/42
摘要： A substantially surface-deactivated catalyst composition that is stable at least to 300° C. The catalyst includes a zeolite catalyst (e.g., ZSM-22, ZSM-23, or ZSM-57) having active internal Brönsted acid sites and a surface-deactivating amount of a rare earth or yttrium oxide (e.g., chosen from lanthanum oxide or lanthanides oxide). This catalyst is preferably used in a process for producing a higher olefin by oligomerizing a light olefin, wherein the process includes contacting a light olefin under oligomerization conditions with the substantially surface-deactivated catalyst composition.
摘要翻译：基本上表面失活的催化剂组合物，其稳定至少为300℃。催化剂包括具有活性内部布朗斯台德酸位点和表面失活的沸石催化剂（例如，ZSM-22，ZSM-23或ZSM-57）稀土或氧化钇的量（例如，选自氧化镧或氧化镧）。该催化剂优选用于通过低聚烯烃生产高级烯烃的方法，其中该方法包括在低聚条件下使轻质烯烃与基本上表面失活的催化剂组合物接触。

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