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11. 发明授权

US06733717B1 Injection stretch-blow molded containers made of olefin polymers 有权
标题翻译：由烯烃聚合物制成的注射拉伸吹塑容器
公开(公告)号：US06733717B1
公开(公告)日：2004-05-11
申请号：US09601356
申请日：2000-08-01
申请人： Bernd Lothar Marczinke , Peter John Vaughan Jones , Meinolf Kersting , David Fischer , Franz Langhauser , Ulrich Moll , Wolfgang Bidell
发明人： Bernd Lothar Marczinke , Peter John Vaughan Jones , Meinolf Kersting , David Fischer , Franz Langhauser , Ulrich Moll , Wolfgang Bidell
IPC分类号： B29C4906
CPC分类号： B29C49/0005 , B29B2911/1402 , B29B2911/14026 , B29B2911/14033 , B29B2911/1404 , B29B2911/14106 , B29B2911/14133 , B29C49/06 , C08F110/06 , C08F210/06 , Y10T428/1352 , C08F2500/12 , C08F2500/15 , C08F2500/03 , C08F210/16
摘要： Injection stretch blow molded containers are obtainable from olefin polymers, comprising homopolymers of propylene or copolymers of propylene with other C2-C10-alk-1-enes, which are obtainable by polymerizing the corresponding monomers with metallocene catalysts. Processes for producing injection stretch blow molded containers from olefin polymers, and also the use of olefin polymers for producing injection stretch blow molded containers, are described.
摘要翻译：注射拉伸吹塑容器可从包含丙烯均聚物或丙烯与其它C 2 -C 10 - 烷-1-烯的共聚物的烯烃聚合物获得，其可通过使金属茂催化剂聚合相应的单体而获得。用于生产注射拉伸吹塑成型描述了烯烃聚合物的容器，以及烯烃聚合物用于生产注射拉伸吹塑容器的用途。

12. 发明授权

US6013742A Process for producing improved random propylene copolymers 失效
标题翻译：制备改进的无规丙烯共聚物的方法
公开(公告)号：US6013742A
公开(公告)日：2000-01-11
申请号：US969278
申请日：1997-11-13
申请人： Stephan Huffer , Meinolf Kersting , Franz Langhauser , Rainer Alexander Werner , Patrik Muller , Jurgen Kerth
发明人： Stephan Huffer , Meinolf Kersting , Franz Langhauser , Rainer Alexander Werner , Patrik Muller , Jurgen Kerth
IPC分类号： C08F4/658 , C08F4/02 , C08F4/64 , C08F4/654 , C08F210/06 , C08F210/16 , D01F6/06 , C08F4/18
CPC分类号： C08F210/16 , C08F210/06
摘要： A process for preparing random propylene copolymers containing copolymerized C.sub.2 -C.sub.10 -alk-1-enes by polymerization of propylene and C.sub.2 -C.sub.10 -alk-1-enes in the presence of a Ziegler-Natta catalyst system comprising a titanium-containing solid component a) comprising a compound of magnesium, a halogen, silica gel as support and a carboxylic ester as electron donor compound, and also, as cocatalysts, an aluminum compound b) and a further electron donor compound c), where propylene and the C.sub.2 -C.sub.10 -alk-1-enes are polymerized with one another at from 50 to 100.degree. C. at pressures in the range from 15 to 40 bar and mean residence times of from 0.5 to 5 hours and the support used in the titanium-containing solid component is a silica gel which has a mean particle diameter of from 5 to 200 .mu.m, a mean particle diameter of the primary particles of from 1 to 10 .mu.m and voids or channels having a mean diameter of from 1 to 10 .mu.m, which voids or channels have a macroscopic proportion by volume based on the total particle in the range from 5 to 20%.
摘要翻译：在含有含钛固体组分a的齐格勒 - 纳塔催化剂体系存在下，通过丙烯和C 2 -C 10 - 烷-1-烯的聚合制备含共聚的C 2 -C 10 - 烷-1-烯的无规丙烯共聚物的方法），其包含镁，卤素，硅胶作为载体的化合物和作为电子给体化合物的羧酸酯，以及作为助催化剂的铝化合物b）和另外的电子给体化合物c），其中丙烯和C 2 -C 10 α-烷-1-烯在50至100℃下以15至40巴的压力和0.5至5小时的平均停留时间彼此聚合，并且在含钛固体组分中使用的载体是平均粒径为5〜200μm，一次粒子的平均粒径为1〜10μm，平均粒径为1〜10μm的通道的硅胶，其中，空隙或通道具有基于体积的宏观比例总颗粒在5至20％的范围内。

13. 发明申请

US20050085610A1 Random propylene copolymers 有权
公开(公告)号：US20050085610A1
公开(公告)日：2005-04-21
申请号：US10971080
申请日：2004-10-25
申请人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Gunther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schone , Meinolf Kersting
发明人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Gunther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schone , Meinolf Kersting
IPC分类号： C08F2/34 , C08F4/02 , C08F4/658 , C08F210/06 , C08F210/16 , D01F6/30 , C08F8/00
CPC分类号： D01F6/30 , C08F210/06 , C08F210/16 , Y10T428/31938 , C08F4/6546 , C08F210/08 , C08F2500/12
摘要： Random copolymers of propylene with other 1-alkenes having up to carbon atoms, whose content of comonomers is in the range from 0.7 to 1.4% by weight if the only comonomer present in the propylene copolymers is ethylene, or whose content of comonomers is in the range from 0.7 to 3.0% by weight if at least one C4-C10-1-alkene is present as comonomer, and whose cold-xylene-soluble fraction is from 1.0 to 2.5% by weight if ethylene is present as a comonomer in the propylene copolymers, or whose cold-xylene-soluble fraction is from 0.75 to 2.0% by weight if the only comonomers present are C4-C10-1-alkenes, and a process for preparing the random copolymers of propylene is described, as is their use for producing films, fibers or moldings, and also the films, fibers and moldings themselves and biaxially stretched films made from random propylene copolymers of this type and processes for their production.

14. 发明申请

US20050085609A1 Random propylene copolymers 有权
标题翻译：无规丙烯共聚物
公开(公告)号：US20050085609A1
公开(公告)日：2005-04-21
申请号：US10971079
申请日：2004-10-25
申请人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Gunther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schone , Meinolf Kersting
发明人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Gunther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schone , Meinolf Kersting
IPC分类号： C08F2/34 , C08F4/02 , C08F4/658 , C08F210/06 , C08F210/16 , D01F6/30 , C08F110/00
CPC分类号： D01F6/30 , C08F210/06 , C08F210/16 , Y10T428/31938 , C08F4/6546 , C08F210/08 , C08F2500/12
摘要： Random copolymers of propylene with other 1-alkenes having up to carbon atoms, whose content of comonomers is in the range from 0.7 to 1.4% by weight if the only comonomer present in the propylene copolymers is ethylene, or whose content of comonomers is in the range from 0.7 to 3.0% by weight if at least one C4-C10-1-alkene is present as comonomer, and whose cold-xylene-soluble fraction is from 1.0 to 2.5% by weight if ethylene is present as a comonomer in the propylene copolymers, or whose cold-xylene-soluble fraction is from 0.75 to 2.0% by weight if the only comonomers present are C4-C10-1-alkenes, and a process for preparing the random copolymers of propylene is described, as is their use for producing films, fibers or moldings, and also the films, fibers and moldings themselves and biaxially stretched films made from random propylene copolymers of this type and processes for their production.
摘要翻译：丙烯与具有至多碳原子的其它1-烯烃的无规共聚物，如果丙烯共聚物中存在的共聚单体中唯一的共聚单体为共聚单体，其共聚单体的含量为0.7-1.4重量％，或其共聚单体的含量为如果至少一个C 4 -C 10 - 1-烯烃作为共聚单体存在，其冷二甲苯可溶成分为如果乙烯作为丙烯共聚物中的共聚单体存在，则其重量为1.0至2.5重量％，或者如果仅存在共聚单体为C 4 - 4，则冷二甲苯可溶成分为0.75-2.0重量％描述了用于制备膜，纤维或模制品的方法，以及薄膜，纤维和模制品本身以及双轴的方法制备丙烯的无规共聚物的方法。由这种类型的无规丙烯共聚物制成的拉伸薄膜及其生产方法。

15. 发明授权

US07026421B2 Random propylene copolymers 有权
标题翻译：无规丙烯共聚物
公开(公告)号：US07026421B2
公开(公告)日：2006-04-11
申请号：US10971079
申请日：2004-10-25
申请人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Günther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schöne , Meinolf Kersting
发明人： David Appleyard , Franz Langhauser , Murray Horton , Roland Hingmann , Günther Schweier , Volker Rauschenberger , Ingolf Hennig , Dieter Lilge , Werner Schöne , Meinolf Kersting
IPC分类号： C08F210/06 , C08F210/08
CPC分类号： D01F6/30 , C08F210/06 , C08F210/16 , Y10T428/31938 , C08F4/6546 , C08F210/08 , C08F2500/12
摘要： Random copolymers of propylene with other 1-alkenes having up to carbon atoms, whose content of comonomers is in the range from 0.7 to 1.4% by weight if the only comonomer present in the propylene copolymers is ethylene, or whose content of comonomers is in the range from 0.7 to 3.0% by weight if at least one C4–C10-1-alkene is present as comonomer, and whose cold-xylene-soluble fraction is from 1.0 to 2.5% by weight if ethylene is present as a comonomer in the propylene copolymers, or whose cold-xylene-soluble fraction is from 0.75 to 2.0% by weight if the only comonomers present are C4–C10-1-alkenes, and a process for preparing the random copolymers of propylene is described, as is their use for producing films, fibers or moldings, and also the films, fibers and moldings themselves and biaxially stretched films made from random propylene copolymers of this type and processes for their production.
摘要翻译：丙烯与具有至多碳原子的其它1-烯烃的无规共聚物，如果丙烯共聚物中存在的共聚单体中唯一的共聚单体为共聚单体，其共聚单体的含量为0.7-1.4重量％，或其共聚单体的含量为如果至少一个C 4 -C 10 - 1-烯烃作为共聚单体存在，其冷二甲苯可溶成分为如果乙烯作为丙烯共聚物中的共聚单体存在，则其重量为1.0至2.5重量％，或者如果仅存在共聚单体为C 4 - 4，则冷二甲苯可溶成分为0.75-2.0重量％描述了用于制备膜，纤维或模制品的方法，以及薄膜，纤维和模制品本身以及双轴的方法制备丙烯的无规共聚物的方法。由这种类型的无规丙烯共聚物制成的拉伸薄膜及其生产方法。

16. 发明授权

US06221984B1 Random propylene copolymer 失效
标题翻译：无规丙烯共聚物
公开(公告)号：US06221984B1
公开(公告)日：2001-04-24
申请号：US09082056
申请日：1998-05-21
申请人： Meinolf Kersting , Werner Schöne , Franz Langhauser
发明人： Meinolf Kersting , Werner Schöne , Franz Langhauser
IPC分类号： C08F444
CPC分类号： C08F10/00 , C08F210/06 , C08F210/16 , Y10S526/916 , C08F4/6546 , C08F2/34 , C08F210/08 , C08F2500/26
摘要： Random copolymers of propylene with ethylene and at least one C4-C10-alk-1-ene, having a melting point, determined by the DSC method, of less than or equal to 135° C., are obtainable by polymerization of propylene, ethylene and at least one C4-C10-alk-1-ene in the absence of a liquid reaction medium from the gas phase at from 50 to 100° C. and a pressure of from 15 to 40 bar in the presence of a Ziegler-Natta catalyst system comprising a) a titanium-containing solid component comprising at least one halogen-containing magnesium compound, an electron donor and an inorganic oxide as support, b) an aluminum compound and c) a further electron donor compound, wherein the ratio of the partial pressures of propylene and ethylene is set to from 20:1 to 100:1 and the ratio of the partial pressures of the C4-C10-alk-1-ene(s) and ethylene is set to from 2.5:1 to 20:1. A process for preparing such random copolymers is also provided, and they can be used in films, fibers or moldings.
摘要翻译：丙烯与乙烯和至少一种具有小于或等于135℃测定的熔点的C4-C10-烷-1-烯的无规共聚物可以通过丙烯，乙烯和在不存在来自气相的液体反应介质的情况下的至少一种C 4 -C 10 - 烷-1-烯在50至100℃和15至40巴的压力下，在齐格勒 - 纳塔催化剂体系包括a）含有至少一种含卤素的镁化合物，电子给体和作为载体的无机氧化物的含钛固体组分，b）铝化合物和c）另外的电子给体化合物，其中分压比的丙烯和乙烯的比例设定为20:1至100:1，并且C4-C10-烷-1-烯和乙烯的分压比设定为2.5:1至20:1。还提供了制备这种无规共聚物的方法，它们可以用于膜，纤维或模制品中。

17. 发明申请

US20100069586A1 HIGH ACTIVITY ZIEGLER-NATTA CATALYSTS, PROCESS FOR PRODUCING CATALYSTS AND USE THEREOF 审中-公开
标题翻译：高活性ZIEGLER-NATTA催化剂，生产催化剂的方法及其用途
公开(公告)号：US20100069586A1
公开(公告)日：2010-03-18
申请号：US12482309
申请日：2009-06-10
申请人： Douglas D. Klendworth , Kenneth W. Johnson , Andreas Winter , Franz Langhauser
发明人： Douglas D. Klendworth , Kenneth W. Johnson , Andreas Winter , Franz Langhauser
IPC分类号： C08F4/50 , C08F4/10
CPC分类号： C08F110/06 , C08F2500/12 , C08F2500/18 , C08F2500/24 , C08F4/6543 , C08F4/651
摘要： Improved Ziegler-Natta catalysts and methods of making the improved catalyst are described. The Ziegler-Natta catalyst is formed using a spherical MgCl2-xROH support, where R is a linear, cyclic or branched hydrocarbon unit with 1-10 carbon atoms and where ROH is an alcohol or a mixture of at least two different alcohols and where x has a range of about 1.5 to 6.0, preferably about 2.5 to 4, more preferably about 2.9 to 3.4, and even more preferably 2.95 to 3.35. The Ziegler-Natta catalyst includes a Group 4-8 transition metal and an internal donor. The catalyst has improved activity in olefin polymerization reactions as well as good stereoregularity and hydrogen sensitivity.
摘要翻译：描述了改进的齐格勒 - 纳塔催化剂和制备改进的催化剂的方法。齐格勒 - 纳塔催化剂使用球形MgCl 2 -xROH载体形成，其中R是具有1-10个碳原子的直链，环状或支链烃单元，其中ROH是醇或至少两种不同醇的混合物，其中x 具有约1.5至6.0，优选约2.5至4，更优选约2.9至3.4，甚至更优选2.95至3.35的范围。齐格勒 - 纳塔催化剂包括4-8族过渡金属和内部供体。催化剂具有改进的烯烃聚合反应活性以及良好的立构规整性和氢敏感性。

18. 发明申请

US20070082806A1 Metallocene catalysts, their synthesis and their use for the polymerization of olefins 审中-公开
公开(公告)号：US20070082806A1
公开(公告)日：2007-04-12
申请号：US11634653
申请日：2006-12-06
申请人： Nicola Paczkowski , Andreas Winter , Franz Langhauser
发明人： Nicola Paczkowski , Andreas Winter , Franz Langhauser
IPC分类号： C08F4/02
CPC分类号： C08F210/06 , C08F4/65912 , C08F4/65916 , C08F4/65927 , C08F210/16 , C08F2500/12 , C08F2500/03
摘要： A process for the preparation of a catalyst system includes the steps of combining a support material with a first composition which includes at least one aluminoxane in a first solvent to provide an aluminoxane loaded support; and, contacting the aluminoxane loaded support with a second composition which includes at least one metallocene compound, a second solvent, and a cocatalyst, wherein the cocatalyst includes a second portion of the at least one aluminoxane alone or in combination with an ionic compound and/or a Lewis acid.

19. 发明申请

US20060116490A1 Metallocene catalysts, their synthesis and their use for the polymerization of olefins 有权
标题翻译：茂金属催化剂，它们的合成及其在烯烃聚合中的应用
公开(公告)号：US20060116490A1
公开(公告)日：2006-06-01
申请号：US11001272
申请日：2004-12-01
申请人： Nicola Paczkowski , Andreas Winter , Franz Langhauser
发明人： Nicola Paczkowski , Andreas Winter , Franz Langhauser
IPC分类号： C08F4/44 , B01J31/00
CPC分类号： C08F210/06 , C08F4/65912 , C08F4/65916 , C08F4/65927 , C08F210/16 , C08F2500/12 , C08F2500/03
摘要： A process for the preparation of a catalyst system includes the steps of combining a support material with a first composition which includes at least one aluminoxane in a first solvent to provide an aluminoxane loaded support; and, contacting the aluminoxane loaded support with a second composition which includes at least one metallocene compound, a second solvent, and a cocatalyst, wherein the cocatalyst includes a second portion of the at least one aluminoxane alone or in combination with an ionic compound and/or a Lewis acid.
摘要翻译：制备催化剂体系的方法包括以下步骤：将载体材料与第一组合物组合，所述第一组合物在第一溶剂中包含至少一种铝氧烷以提供负载铝氧烷的载体; 并且使含有铝氧烷的载体与包含至少一种茂金属化合物，第二溶剂和助催化剂的第二组合物接触，其中助催化剂包括单独的至少一种铝氧烷的第二部分或与离子化合物和/ 或路易斯酸。

20. 发明授权

US06593442B2 Semicrystalline propylene polymer compositions with good suitability for producing biaxially oriented films 有权
标题翻译：具有良好适用于生产双轴取向膜的半结晶丙烯聚合物组合物
公开(公告)号：US06593442B2
公开(公告)日：2003-07-15
申请号：US09737848
申请日：2000-12-18
申请人： Wolfgang Bidell , Roland Hingmann , Franz Langhauser , Dieter Lilge , Volker Rauschenberger , Günther Schweier , Florian Stricker , Jürgen Suhm
发明人： Wolfgang Bidell , Roland Hingmann , Franz Langhauser , Dieter Lilge , Volker Rauschenberger , Günther Schweier , Florian Stricker , Jürgen Suhm
IPC分类号： C08F1006
CPC分类号： C08F297/08 , C08F4/65904 , C08F4/65908 , C08F4/65916 , C08F10/06 , C08F110/06 , C08F210/06 , C08L23/14 , C08L2205/02 , C08L2314/06 , Y10S264/901 , Y10S428/91 , Y10S526/905 , C08F4/65927 , C08F2/001 , C08L2666/04 , C08F2500/26 , C08F210/16
摘要： A semicrystalline propylene polymer composition with good suitability for producing biaxially oriented films and prepared by polymerizing propylene, ethylene and/or C4-C18-1-alkenes, where at least 50 mol % of the monomer units present arise from the polymerization of propylene. Also described is the use of the semicrystalline propylene polymer composition for producing films, fibers or moldings, the films, fibers and moldings made from these compositions, biaxially stretched films made from the semicrystalline propylene polymer compositions, and also a method for characterizing the semicrystalline propylene polymer compositions.
摘要翻译：一种半结晶丙烯聚合物组合物，其具有良好的适用于生产双轴取向薄膜并通过聚合丙烯，乙烯和/或C 4 -C 18 -1-烯烃制备，其中存在至少50摩尔％的单体单元来自丙烯的聚合。还描述了使用半结晶丙烯聚合物组合物来生产膜，纤维或模制品，由这些组合物制成的膜，纤维和模制品，由半结晶丙烯聚合物组合物制成的双轴向拉伸膜，以及用于表征半结晶丙烯聚合物组合物。

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