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11. 发明授权

US07501195B2 Drive control of power system including fuel cells 失效
标题翻译：电力系统的驱动控制，包括燃料电池
公开(公告)号：US07501195B2
公开(公告)日：2009-03-10
申请号：US10826367
申请日：2004-04-19
申请人： Satoshi Aoyama , Shigeru Ogino , Yasuhiro Izawa , Satoshi Iguchi , Takatoshi Masui
发明人： Satoshi Aoyama , Shigeru Ogino , Yasuhiro Izawa , Satoshi Iguchi , Takatoshi Masui
IPC分类号： H01M8/18 , H01M8/04 , H01M8/12
CPC分类号： H01M8/04753 , B60L11/1885 , H01M8/04231 , H01M8/0432 , H01M8/04373 , H01M8/04947 , H01M8/0612 , H01M16/006 , Y02T90/34
摘要： A power system of the invention includes fuel cells and a fuel gas generation system that generates a fuel gas to be supplied to the fuel cells. At the time of stopping supply of hydrogen, the fuel gas generation system selectively uses a stop process that replaces hydrogen in a hydrogen separator unit with the air for removal of hydrogen and a pause process that allows hydrogen to remain in the hydrogen separator unit. The stop process is selected when the fuel gas generation system stops the supply of hydrogen for a long time period. The pause process is selected when the fuel gas generation system temporarily stops the supply of hydrogen. The arrangement of the invention desirably shortens a restart time of the fuel gas generation system and reduces a potential energy loss.
摘要翻译：本发明的电力系统包括燃料电池和产生要供应到燃料电池的燃料气体的燃料气体生成系统。在停止供给氢时，燃料气体发生系统选择性地使用用氢气分离器单元中的氢替代用于除去氢的空气的停止过程和允许氢保留在氢分离器单元中的暂停过程。当燃料气体发生系统长时间停止供氢时，选择停止过程。当燃气生成系统暂时停止供氢时，选择暂停处理。本发明的装置期望地缩短了燃料气体发生系统的重新启动时间并且减少了潜在的能量损失。

12. 发明授权

US07255721B1 Device forming fuel gas for fuel cell and composite material for hydrogen separation 失效
标题翻译：用于燃料电池的装置形成燃料气体和用于氢气分离的复合材料
公开(公告)号：US07255721B1
公开(公告)日：2007-08-14
申请号：US10130063
申请日：2000-11-09
申请人： Hiromichi Sato , Satoshi Iguchi , Toshihide Nakata , Satoshi Aoyama
发明人： Hiromichi Sato , Satoshi Iguchi , Toshihide Nakata , Satoshi Aoyama
IPC分类号： C10L5/00 , B01D53/22
CPC分类号： B01D69/145 , B01D53/228 , B01D53/864 , B01D67/0069 , B01D67/0072 , B01D69/10 , B01D69/141 , B01D71/02 , B01D71/022 , B01D2325/06 , B01D2325/10 , B01J8/009 , B01J12/007 , B01J19/2425 , B01J19/2475 , B01J19/2485 , B01J2208/00849 , B01J2219/00137 , B01J2219/1944 , B01J2219/1945 , C01B3/38 , C01B3/40 , C01B3/503 , C01B3/505 , C01B2203/0233 , C01B2203/0283 , C01B2203/041 , C01B2203/044 , C01B2203/047 , C01B2203/0495 , C01B2203/066 , C01B2203/0883 , C01B2203/0894 , C01B2203/1011 , C01B2203/1023 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1223 , C01B2203/1241 , C01B2203/1276 , C01B2203/1288 , C01B2203/146 , C01B2203/80 , C01B2203/82 , H01M4/94 , H01M8/0612 , H01M8/0662 , Y02P20/149 , Y02P20/52 , Y02P70/56 , Y10S55/05
摘要： For a reforming device that generates fuel gas for fuel cells by decomposing hydrocarbon compounds such as natural gas and then using a hydrogen separation composite to selectively transmit hydrogen, a hydrogen separation composite having the following structure is used. A porous support medium made of ceramics, etc. is formed, and a hydrogen separation metal is supported in the pores so as to fill the inside of the support medium. It is also possible to support a reforming catalyst. By doing this, it is possible to increase the area at which the hydrogen separation metal contacts gas, so the hydrogen transmission performance is increased. Furthermore, to prevent raw material gas leaks due to pin holes, high pressure gas is supplied to the hydrogen extraction side, and the total pressure is made higher than the pressure on the raw material gas supply side without making the hydrogen partial pressure higher. By using these means, it is possible to increase the hydrogen separation performance for the reforming device and to make the device more compact.
摘要翻译：对于通过分解诸如天然气的烃化合物然后使用氢分离复合物来选择性地传输氢而产生用于燃料电池的燃料气体的重整装置，使用具有以下结构的氢分离复合材料。形成由陶瓷等制成的多孔载体介质，并将氢分离金属负载在孔中以填充载体介质的内部。还可以负载重整催化剂。通过这样做，可以增加氢分离金属与气体接触的面积，从而提高氢气传输性能。此外，为了防止原料气体由于针孔泄漏，向氢气提取侧供给高压气体，使总压力高于原料气体供给侧的压力，而不会使氢分压变高。通过这些方法，可以提高重整装置的氢分离性能，并且使装置更紧凑。

13. 发明授权

US06656617B2 Fuel gas production system for fuel cells 失效
标题翻译：燃料电池燃气生产系统
公开(公告)号：US06656617B2
公开(公告)日：2003-12-02
申请号：US09758387
申请日：2001-01-12
申请人： Satoshi Aoyama , Hiromichi Sato , Toshihide Nakata , Satoshi Iguchi
发明人： Satoshi Aoyama , Hiromichi Sato , Toshihide Nakata , Satoshi Iguchi
IPC分类号： H01M804
CPC分类号： H01M8/2483 , C01B3/384 , C01B3/48 , C01B3/505 , C01B2203/0233 , C01B2203/0283 , C01B2203/041 , C01B2203/044 , C01B2203/047 , C01B2203/066 , C01B2203/1076 , H01M8/0258 , H01M8/0267 , H01M8/04223 , H01M8/04225 , H01M8/04268 , H01M8/0631 , H01M8/0662 , H01M8/0668 , H01M8/0687
摘要： The technique of the present invention enhances the separation efficiency and the production efficiency of hydrogen in a hydrogen production system for fuel cells, while reducing the size of the whole fuel gas production system. In the fuel gas production system of the present invention, a hydrocarbon compound is subjected to multi-step chemical processes including a reforming reaction, a shift reaction, and a CO oxidation to give a hydrogen-rich fuel gas. Gaseous hydrogen produced through the reforming reaction is separated by a hydrogen separation membrane having selective permeability to hydrogen. The residual gas after the separation of hydrogen has a low hydrogen partial pressure and undergoes the shift reaction at the accelerated rate. The hydrogen-rich processed gas obtained through the shift reaction and the CO oxidation joins with the separated hydrogen and is supplied to fuel cells. A purge gas for carrying out the hydrogen is introduced into a separation unit of hydrogen, in order to lower the hydrogen partial pressure and thereby enhance the separation efficiency of hydrogen. The residual gas after the separation of hydrogen undergoes combustion and is subsequently used as the purge gas
摘要翻译：本发明的技术提高了燃料电池的氢生产系统中的氢的分离效率和生产效率，同时减小了整个燃料气体生产系统的尺寸。在本发明的燃料气体生产系统中，烃化合物进行包括重整反应，转移反应和CO氧化在内的多步化学处理，得到富氢燃料气体。通过重整反应产生的气态氢气通过对氢具有选择性渗透性的氢分离膜分离。氢分离后的残留气体具有低的氢分压，并以加速速率进行转化反应。通过转移反应和CO氧化获得的富氢处理气体与分离的氢气连接并供应到燃料电池。用于进行氢气的吹扫气体被引入到氢的分离单元中，以便降低氢气分压，从而提高氢的分离效率。氢气分离后的残余气体经历燃烧，随后用作净化气体

14. 发明申请

US20080145726A1 Hydrogen-Generating Apparatus and Fuel Cell System 失效
标题翻译：氢发生装置和燃料电池系统
公开(公告)号：US20080145726A1
公开(公告)日：2008-06-19
申请号：US11883163
申请日：2006-03-08
申请人： Keisuke Nagasaka , Naoki Ito , Satoshi Iguchi , Satoshi Aoyama , Hiroshi Aoki , Takashi Shimazu , Hiroyuki Mitsui
发明人： Keisuke Nagasaka , Naoki Ito , Satoshi Iguchi , Satoshi Aoyama , Hiroshi Aoki , Takashi Shimazu , Hiroyuki Mitsui
IPC分类号： H01M8/18
CPC分类号： B60L11/1898 , B60L11/1892 , C01B3/46 , C01B2203/066 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , H01M8/04007 , H01M8/0612 , Y02P20/128 , Y02T90/34
摘要： The present invention provides a hydrogen-generating apparatus comprising two catalytic reactors cyclically operating reforming and regeneration (combustion) mode, in which the reduction in reforming efficiency associated with an increase in switching frequency to the regeneration reaction can be suppressed, and generation of hydrogen by reforming can stably be performed. In the reforming reaction, a cathode offgas discharged from a hydrogen-separation-membrane fuel cell 30 having a hydrogen-permeating film is supplied to PSR reformers 10 and 20, in which the reforming reaction and the regeneration reaction are performed alternately.
摘要翻译：本发明提供了一种氢发生装置，其包括循环运行的重整和再生（燃烧）模式的两个催化反应器，其中可以抑制与再生反应的开关频率的增加相关的重整效率的降低，以及通过可以稳定地进行重整。在重整反应中，从具有氢渗透膜的氢分离膜燃料电池30排出的阴极废气被供给到重整反应和再生反应交替进行的PSR重整器10和20中。

15. 发明授权

US08382864B2 Hydrogen-generating apparatus and fuel cell system 失效
标题翻译：氢发生装置和燃料电池系统
公开(公告)号：US08382864B2
公开(公告)日：2013-02-26
申请号：US11883163
申请日：2006-03-08
申请人： Keisuke Nagasaka , Naoki Ito , Satoshi Iguchi , Satoshi Aoyama , Hiroshi Aoki , Takashi Shimazu , Hiroyuki Mitsui
发明人： Keisuke Nagasaka , Naoki Ito , Satoshi Iguchi , Satoshi Aoyama , Hiroshi Aoki , Takashi Shimazu , Hiroyuki Mitsui
IPC分类号： B01J8/00
CPC分类号： B60L11/1898 , B60L11/1892 , C01B3/46 , C01B2203/066 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , H01M8/04007 , H01M8/0612 , Y02P20/128 , Y02T90/34
摘要： The present invention provides a hydrogen-generating apparatus in which the reduction in reforming efficiency associated with an increase in switching frequency to the regeneration reaction can be suppressed, and generation of hydrogen by reforming can stably be performed. In the reforming reaction, a cathode offgas discharged from a hydrogen-separation-membrane fuel cell 30 having a hydrogen-permeating film is supplied to PSR reformers 10 and 20, in which the reforming reaction and the regeneration reaction are performed alternately.
摘要翻译：本发明提供一种氢发生装置，其中可以抑制与再生反应的开关频率的增加相关的重整效率的降低，并且可以稳定地进行通过重整产生的氢。在重整反应中，从具有氢渗透膜的氢分离膜燃料电池30排出的阴极废气被供给到重整反应和再生反应交替进行的PSR重整器10和20中。

16. 发明申请

US20080138679A1 Hydrogen Generation Device and Fuel Cell System Including Same 审中-公开
标题翻译：氢发生装置和包括燃料电池系统的燃料电池系统
公开(公告)号：US20080138679A1
公开(公告)日：2008-06-12
申请号：US11885670
申请日：2006-04-04
申请人： Masahiko Iijima , Satoshi Iguchi , Satoshi Shiokawa
发明人： Masahiko Iijima , Satoshi Iguchi , Satoshi Shiokawa
IPC分类号： H01M8/18
CPC分类号： H01M8/126 , C01B3/38 , C01B3/46 , C01B2203/0233 , C01B2203/0283 , C01B2203/0445 , C01B2203/047 , C01B2203/049 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/1023 , C01B2203/1247 , C01B2203/127 , H01M4/94 , H01M8/04007 , H01M8/04223 , H01M8/04225 , H01M8/0618 , H01M8/0662 , H01M8/1246 , Y02E60/525 , Y02P20/128 , Y02P70/56
摘要： A hydrogen generation device includes a catalyst; a sulfur-trap member; a soot-trap member; a pair of reformers; and a control portion. In each reformer, a reforming reaction is carried out to generate hydrogen-containing gas using gasoline and cathode off-gas on the catalyst, and an exothermic reaction is carried out to heat the catalyst using anode off-gas and air. The control portion executes a control such that the reactant and the exothermic material are alternately supplied to each reformer, whereby the reforming reaction and the exothermic reaction are alternately carried out in each reformer. A fuel cell system includes the hydrogen generation device.
摘要翻译：氢生成装置包括催化剂; 硫捕集器; 烟炱捕捉器; 一对改革者和控制部。在每个重整器中，进行重整反应以在催化剂上使用汽油和阴极废气产生含氢气体，并且进行放热反应以使用阳极废气和空气加热催化剂。控制部执行将反应物和放热材料交替供给至各重整器的控制，由此在各重整器中交替进行重整反应和放热反应。燃料电池系统包括氢气生成装置。

17. 发明申请

US20070248872A1 Membrane-Electrode Assembly and Fuel Cell 有权
标题翻译：膜 - 电极组件和燃料电池
公开(公告)号：US20070248872A1
公开(公告)日：2007-10-25
申请号：US11659539
申请日：2005-08-17
申请人： Satoshi Aoyama , Satoshi Iguchi , Makoto Taniguchi
发明人： Satoshi Aoyama , Satoshi Iguchi , Makoto Taniguchi
IPC分类号： B01J21/18 , H01M4/00
CPC分类号： C01B3/501 , C01B2203/0405 , H01M4/9033 , H01M4/9041 , H01M4/94 , H01M8/0232 , H01M8/0267 , H01M8/0297 , H01M8/241 , H01M8/2457 , H01M8/2483 , H01M2008/1293
摘要： An electrolyte layer (121) and a hydrogen-permeable metal layer (122) are fitted in a fitting portion (131) of a low thermal expansion member (130), and a cathode electrode (110) is provided on the electrolyte layer (121). Gas separators (100, 150) are provided such that a low thermal expansion member (130) is held between the gas separators (100, 150). Since the low thermal expansion member (130) is made of metal which has a thermal expansion coefficient lower than that of the hydrogen-permeable metal layer (122), thermal expansion of the hydrogen-permeable metal layer (122) can be suppressed. Accordingly, it is possible to reduce shear stress applied to an interface between the electrolyte layer (121) and the hydrogen-permeable metal layer (122) due to the thermal expansion. It is possible to suppress separation of the electrolyte layer (121) from the hydrogen-permeable metal layer (122) and occurrence of a crack in the electrolyte layer (121).
摘要翻译：电解质层（121）和透氢性金属层（122）嵌合在低热膨胀构件（130）的嵌合部（131）中，阴极电极（110）设置在电解质层）。气体分离器（100,150）被设置成使得低热膨胀构件（130）保持在气体分离器（100,150）之间。由于低热膨胀构件（130）由热膨胀系数低于透氢性金属层（122）的热膨胀系数的金属制成，所以可以抑制透氢性金属层（122）的热膨胀。因此，由于热膨胀，可以减少施加到电解质层（121）和氢可渗透金属层（122）之间的界面的剪切应力。可以抑制电解质层（121）与透氢性金属层（122）的分离，并且在电解质层（121）中产生裂纹。

18. 发明授权

US06811578B2 Fuel reforming apparatus and method of controlling same 失效
标题翻译：燃料重整装置及其控制方法
公开(公告)号：US06811578B2
公开(公告)日：2004-11-02
申请号：US09976111
申请日：2001-10-15
申请人： Kazuhisa Kunitake , Satoshi Iguchi , Satoshi Aoyama , Hiroyuki Usami
发明人： Kazuhisa Kunitake , Satoshi Iguchi , Satoshi Aoyama , Hiroyuki Usami
IPC分类号： B01J802
CPC分类号： B60L11/1892 , B01J2219/00191 , B60L11/1885 , B60L11/1887 , B60L11/1894 , B60L2200/26 , C01B3/323 , C01B3/382 , C01B3/48 , C01B2203/0244 , C01B2203/0283 , C01B2203/044 , C01B2203/047 , C01B2203/066 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/0844 , C01B2203/085 , C01B2203/0866 , C01B2203/0883 , C01B2203/1041 , C01B2203/1082 , C01B2203/1247 , C01B2203/1276 , C01B2203/1288 , C01B2203/16 , C01B2203/1604 , C01B2203/1619 , C01B2203/1661 , C01B2203/1685 , C01B2203/169 , C01B2203/1695 , C01B2203/82 , H01M8/0612 , H01M8/0618 , H01M2250/20 , Y02P20/128 , Y02T90/32 , Y02T90/34
摘要： In a fuel reforming apparatus having a reformer for reforming a raw fuel containing a hydrocarbon-containing compound so as to produce a hydrogen-rich fuel gas for use in a fuel cell, a carbon removal process for removing carbon deposited on a reforming catalyst contained in the reformer is executed by controlling the amount of the raw fuel supplied to the reformer and the amount of the oxygen supplied to the reformer so that a ratio of the number of oxygen atoms O supplied to the reformer to the number of carbon atoms supplied to the reformer becomes larger than an appropriate range of the O/C ratio that is to be established during a normal operation of the reformer.
摘要翻译：在具有用于重整含有含烃化合物的原料燃料以便产生用于燃料电池的富氢燃料气体的重整器的燃料重整装置中，除去沉积在包含在重整催化剂中的重整催化剂上的碳通过控制供给到重整器的原料燃料的量和向重整器供给的氧气的量来控制重整器，使得供给至重整器的氧原子数O与供给至重整器的碳原子数之比重整器变得大于在重整器的正常操作期间建立的O / C比的适当范围。

19. 发明授权

US06783877B2 Fuel reforming apparatus 失效
标题翻译：燃料重整装置
公开(公告)号：US06783877B2
公开(公告)日：2004-08-31
申请号：US09930989
申请日：2001-08-17
申请人： Takashi Shimazu , Satoshi Iguchi , Satoshi Aoyama , Koichi Numata , Kazuhisa Kunitake , Takeshi Nishikawa , Shuichi Kubo , Satoshi Yamazaki
发明人： Takashi Shimazu , Satoshi Iguchi , Satoshi Aoyama , Koichi Numata , Kazuhisa Kunitake , Takeshi Nishikawa , Shuichi Kubo , Satoshi Yamazaki
IPC分类号： H01M804
CPC分类号： H01M8/0612 , B01B1/005 , B01J19/0006 , B01J19/0013 , B01J19/0026 , B01J19/088 , B01J19/2485 , B01J19/26 , B01J2208/00716 , B01J2219/00006 , B01J2219/00063 , B01J2219/00087 , B01J2219/00117 , B01J2219/00123 , B01J2219/00157 , B01J2219/00159 , B01J2219/00162 , B01J2219/00164 , B01J2219/00166 , B01J2219/00186 , B01J2219/00198 , B01J2219/00211 , B01J2219/00216 , B01J2219/00218 , B01J2219/00231 , B01J2219/00236 , B01J2219/00247 , B01J2219/0896 , B01J2219/182 , B01J2219/1943 , C01B3/38 , C01B3/382 , C01B3/48 , C01B3/583 , C01B2203/0233 , C01B2203/0244 , C01B2203/0261 , C01B2203/0277 , C01B2203/0283 , C01B2203/044 , C01B2203/047 , C01B2203/066 , C01B2203/0805 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/0844 , C01B2203/0861 , C01B2203/0866 , C01B2203/0877 , C01B2203/0883 , C01B2203/0894 , C01B2203/1041 , C01B2203/1047 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1247 , C01B2203/127 , C01B2203/1282 , C01B2203/1288 , C01B2203/142 , C01B2203/143 , C01B2203/148 , C01B2203/16 , C01B2203/1604 , C01B2203/1614 , C01B2203/1628 , C01B2203/1657 , C01B2203/1685 , C01B2203/169 , C01B2203/1695 , C01B2203/80 , C01B2203/82 , F01N2240/30 , H01M8/04223 , H01M8/04302 , H01M8/241 , H01M8/2457 , Y02P20/128
摘要： In a fuel cell system 10, a cracking unit 20 is provided upstream of a reformer 36. When the cracking unit 20 is supplied with oxygen and gasoline as a hydrocarbon-based fuel, the gasoline is partially oxidized and decomposed using oxidation-generated heat to give a hydrocarbon with a lower carbon number. The hydrocarbon with the lower carbon number obtained by such gasoline pyrolysis is fed to the reformer 36 and supplied to a reforming reaction zone.
摘要翻译：在燃料电池系统10中，在重整器36的上游设置有裂解装置20.当以裂解装置20供给作为烃类燃料的氧气和汽油时，汽油被氧化生成的热量部分氧化分解，得到碳数较少的烃。通过这种汽油热分解获得的具有较低碳原子数的烃被供给至重整器36并供给至重整反应区。

20. 发明授权

US07718303B2 Membrane-electrode assembly and fuel cell 有权
标题翻译：膜 - 电极组件和燃料电池
公开(公告)号：US07718303B2
公开(公告)日：2010-05-18
申请号：US11659539
申请日：2005-08-17
申请人： Satoshi Aoyama , Satoshi Iguchi , Makoto Taniguchi
发明人： Satoshi Aoyama , Satoshi Iguchi , Makoto Taniguchi
IPC分类号： H01M4/00
CPC分类号： C01B3/501 , C01B2203/0405 , H01M4/9033 , H01M4/9041 , H01M4/94 , H01M8/0232 , H01M8/0267 , H01M8/0297 , H01M8/241 , H01M8/2457 , H01M8/2483 , H01M2008/1293
摘要： An electrolyte layer (121) and a hydrogen-permeable metal layer (122) are fitted in a fitting portion (131) of a low thermal expansion member (130), and a cathode electrode (110) is provided on the electrolyte layer (121). Gas separators (100, 150) are provided such that a low thermal expansion member (130) is held between the gas separators (100, 150). Since the low thermal expansion member (130) is made of metal which has a thermal expansion coefficient lower than that of the hydrogen-permeable metal layer (122), thermal expansion of the hydrogen-permeable metal layer (122) can be suppressed. Accordingly, it is possible to reduce shear stress applied to an interface between the electrolyte layer (121) and the hydrogen-permeable metal layer (122) due to the thermal expansion. It is possible to suppress separation of the electrolyte layer (121) from the hydrogen-permeable metal layer (122) and occurrence of a crack in the electrolyte layer (121).
摘要翻译：电解质层（121）和透氢性金属层（122）嵌合在低热膨胀部件（130）的嵌合部（131）中，阴极电极（110）设置在电解质层）。气体分离器（100,150）被设置成使得低热膨胀构件（130）保持在气体分离器（100,150）之间。由于低热膨胀构件（130）由热膨胀系数低于透氢性金属层（122）的热膨胀系数的金属制成，所以可以抑制透氢性金属层（122）的热膨胀。因此，由于热膨胀，可以减少施加到电解质层（121）和氢可渗透金属层（122）之间的界面的剪切应力。可以抑制电解质层（121）与透氢性金属层（122）的分离，并且在电解质层（121）中产生裂纹。

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