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91. 发明申请

US20120241315A1 ELECTROLYSIS DEVICE AND REFRIGERATOR 审中-公开
标题翻译：电解设备和制冷器
公开(公告)号：US20120241315A1
公开(公告)日：2012-09-27
申请号：US13408234
申请日：2012-02-29
申请人： Norihiro Yoshinaga , Yoshihiko Nakano , Norihiro Tomimatsu , Yoshihiro Akasaka
发明人： Norihiro Yoshinaga , Yoshihiko Nakano , Norihiro Tomimatsu , Yoshihiro Akasaka
IPC分类号： C25B9/10 , C25B11/06
CPC分类号： C25B1/30 , C25B9/10 , F25D17/042 , F25D2317/0411
摘要： An electrolysis device of an embodiment includes: an anode, a cathode having a nitrogen-containing carbon alloy catalyst, and an electrolysis cell having a membrane electrode assembly composed of an electrolyte present between the anode and the cathode so that voltage is applied to the anode and the cathode, wherein the electrolyte is any one of acidic, neutral, or alkali, water is produced by the electrolysis device at the cathode, when the electrolyte is acidic, and hydroxide ion is produced by the electrolysis device at the anode, when the electrolyte is neutral or alkali.
摘要翻译：一个实施方案的电解装置包括：阳极，具有含氮碳合金催化剂的阴极和具有由阳极和阴极之间存在的电解质构成的膜电极组件的电解槽，使得电压施加到阳极和阴极，其中电解质是阴极中的电解装置产生的酸性，中性或碱性的任何一种，当电解质为酸性时，在阳极处由电解装置产生氢氧根离子，当电解液是中性或碱。

92. 发明申请

US20120164555A1 COLLECTOR MEMBER, POWER GENERATOR, AND METHOD OF MANUFACTURING COLLECTOR MEMBER FOR POWER GENERATOR 审中-公开
标题翻译：收集器，发电机及其发电机收集器构件的制造方法
公开(公告)号：US20120164555A1
公开(公告)日：2012-06-28
申请号：US13417893
申请日：2012-03-12
申请人： Mutsuki YAMAZAKI , Yoshihiko Nakano , Wu Mei
发明人： Mutsuki YAMAZAKI , Yoshihiko Nakano , Wu Mei
IPC分类号： H01M4/90 , H01M4/92 , B05D5/12 , H01M8/10
CPC分类号： H01M4/8875 , H01M4/8605 , H01M4/8871 , H01M4/921 , H01M4/926 , H01M8/0234 , H01M8/1007 , Y02P70/56
摘要： According to an aspect of the present invention, there is provided a collector member 10 comprising a sheet-shaped base material 11 having a carbon-containing fiber 11a and catalyst particles 12 adhered to an outer periphery of the fiber 11a, containing a noble metal or an alloy thereof, and having an average particle diameter of 0.1 to 2 μm.
摘要翻译：根据本发明的一个方面，提供了一种集电体部件10，其包括具有含碳纤维11a的片状基材11和粘附在纤维11a的外周的催化剂粒子12，其含有贵金属或其合金，平均粒径为0.1〜2μm。

93. 发明授权

US07892694B2 Electrolytic membrane, process for producing the same, membrane electrode assembly, fuel cell and method of operating the same 有权
标题翻译：电解膜，其制造方法，膜电极组件，燃料电池及其操作方法
公开(公告)号：US07892694B2
公开(公告)日：2011-02-22
申请号：US11616565
申请日：2006-12-27
申请人： Yoshihiko Nakano , Hideo Ohta , Kazuhiro Yasuda , Jun Tamura
发明人： Yoshihiko Nakano , Hideo Ohta , Kazuhiro Yasuda , Jun Tamura
IPC分类号： H01M8/10
CPC分类号： C08J9/405 , C08J2425/00 , H01M8/04197 , H01M8/04201 , H01M8/1011 , H01M8/1023 , H01M8/1072 , H01M8/1088 , Y02E60/523 , Y02P70/56
摘要： An electrolytic membrane comprising a porous membrane substrate containing a cross-linked polymer electrolyte having at least a structural component shown by following chemical formula 1: wherein A represents a repeating unit having an aromatic hydrocarbon group substituted by at least a sulfonic acid group, B represents a repeating unit having one of a nitrogen-containing hetero ring compound residue, and the sulfate, hydrochloride or organic sulfonate thereof, C represents a repeating unit having a cross-linked group, and X, Y and Z represent mol fractions of respective repeating units in the chemical formula 1, with 0.34≦X≦0.985, 0.005≦Y≦0.49, 0.01≦Z≦0.495 and Y≦X and Z≦X, provided that, in the repeating unit A, a ratio of the aromatic hydrocarbon group substituted by at least a sulfonic acid group is 0.3 to 1.0, and the number of the sulfonic acid group in the aromatic hydrocarbon group is 1 to 3.
摘要翻译：一种电解质膜，其含有具有至少具有下述化学式1所示的结构成分的交联聚合物电解质的多孔膜基材：其中，A表示具有至少被磺酸基取代的芳香族烃基的重复单元，B表示具有含氮杂环化合物残基和硫酸盐，盐酸盐或其有机磺酸盐之一的重复单元，C表示具有交联基团的重复单元，X，Y和Z表示各个重复单元的摩尔分数在化学式1中，与重复单元A中的芳香族化合物的比例为0.34＆lt; NlE; X＆lt; ll; 0.985,0.005＆lt; 1; Y＆lt; ll; 0.49,0.01和n1E; Z＆lt; NE; 0.495和Y＆由至少磺酸基取代的烃基为0.3〜1.0，芳香族烃基中的磺酸基数为1〜3。

94. 发明授权

US07759277B2 Fuel cell catalyst, process for preparation of the same, and membrane electrode assembly and fuel cell employing the catalyst 有权
标题翻译：燃料电池催化剂，其制备方法以及使用催化剂的膜电极组件和燃料电池
公开(公告)号：US07759277B2
公开(公告)日：2010-07-20
申请号：US12407076
申请日：2009-03-19
申请人： Taishi Fukazawa , Wu Mei , Yoshihiko Nakano , Tsuyoshi Kobayashi , Itsuko Mizutani , Hiroyasu Sumino
发明人： Taishi Fukazawa , Wu Mei , Yoshihiko Nakano , Tsuyoshi Kobayashi , Itsuko Mizutani , Hiroyasu Sumino
IPC分类号： B01J21/00 , H01M4/00
CPC分类号： H01M4/8867 , H01M4/8605 , H01M4/8871 , H01M4/8882 , H01M4/921 , H01M4/926 , H01M8/1007 , Y02P70/56
摘要： The present invention provides a catalyst having high activity and excellent stability, a process for preparation of the catalyst, a membrane electrode assembly, and a fuel cell. The catalyst of the present invention comprises an electronically conductive support and catalyst fine particles. The catalyst fine particles are supported on the support and are represented by the formula (1): PtuRuxGeyTz (1). In the formula, u, x, y and z mean 30 to 60 atm %, 20 to 50 atm %, 0.5 to 20 atm % and 0.5 to 40 atm %, respectively. When the element represented by T is Al, Si, Ni, W, Mo, V or C, the content of the T-element's atoms connected with oxygen bonds is not more than four times as large as that of the T-element's atoms connected with metal bonds on the basis of X-ray photoelectron spectrum (XPS) analysis. When the T-element is Ti, Hf, Sn, Ta, Zr or Nb, the content of the T-element's atoms connected with metal bonds is not more than twice as large as that of the T-element's atoms connected with oxygen bonds on the basis of XPS analysis.
摘要翻译：本发明提供了具有高活性和优异稳定性的催化剂，制备催化剂的方法，膜电极组件和燃料电池。本发明的催化剂包括电子导电载体和催化剂细颗粒。催化剂细颗粒负载在载体上，由式（1）表示：PtuRuxGeyTz（1）。在该式中，u，x，y和z分别表示30〜60atm％，20〜50atm％，0.5〜20atm％，0.5〜40atm％。当由T表示的元素是Al，Si，Ni，W，Mo，V或C时，与氧键连接的T元素原子的含量不超过T元素连接原子的含量的四倍在X射线光电子能谱（XPS）分析的基础上进行金属键合。当T元素是Ti，Hf，Sn，Ta，Zr或Nb时，与金属键连接的T元素原子的含量不超过与氧键连接的T元素原子的含量的两倍 XPS分析的基础。

95. 发明授权

US07759019B2 Liquid fuel cell, membrane electrode assembly and cathode 有权
标题翻译：液体燃料电池，膜电极组件和阴极
公开(公告)号：US07759019B2
公开(公告)日：2010-07-20
申请号：US11370852
申请日：2006-03-09
申请人： Wu Mei , Miho Maruyama , Jun Tamura , Yoshihiro Akasaka , Yoshihiko Nakano
发明人： Wu Mei , Miho Maruyama , Jun Tamura , Yoshihiro Akasaka , Yoshihiko Nakano
IPC分类号： H01M4/00
CPC分类号： H01M4/8605 , H01M4/90 , H01M4/9083 , H01M4/923 , H01M4/926 , H01M8/1011 , Y02E60/523
摘要： A cathode includes a diffusion layer, and a porous catalyst layer provided on the diffusion layer. The porous catalyst layer has a thickness not greater than 60 μm, a porosity of 30 to 70% and a pore diameter distribution including a peak in a range of 20 to 200 nm of a pore diameter. A volume of pores having a diameter of 20 to 200 nm is not less than 50% of a pore volume of the porous catalyst layer. The porous catalyst layer contains a supported catalyst comprising 10 to 30% by weight of a fibrous supported catalyst and 70 to 90% by weight of a granular supported catalyst. The fibrous supported catalyst includes a carbon nanofiber having a herringbone structure or a platelet structure. The granular supported catalyst includes a carbon black having 200 to 600 mL/100 g of a dibutyl phthalate (DBP) absorption value.
摘要翻译：阴极包括扩散层和设置在扩散层上的多孔催化剂层。多孔催化剂层的厚度不大于60μm，孔隙率为30-70％，孔径分布包括孔径在20至200nm范围内的峰。一直径为20〜200nm的孔体积不小于多孔催化剂层的孔体积的50％。多孔催化剂层包含载体催化剂，其包含10至30重量％的纤维负载催化剂和70至90重量％的颗粒负载型催化剂。纤维状载体催化剂包括具有人字形结构或血小板结构的碳纳米纤维。颗粒状载体催化剂包括具有200至600mL / 100g邻苯二甲酸二丁酯（DBP）吸收值的炭黑。

96. 发明申请

US20100003566A1 PROTON-CONDUCTIVE INORGANIC MATERIAL FOR FUEL CELL AND FUEL CELL ANODE EMPLOYING THE SAME 有权
标题翻译：用于燃料电池的导电无机材料和使用它的燃料电池阳极
公开(公告)号：US20100003566A1
公开(公告)日：2010-01-07
申请号：US12302949
申请日：2008-10-03
申请人： Jun Tamura , Yoshihiko Nakano , Yasuhiro Goto
发明人： Jun Tamura , Yoshihiko Nakano , Yasuhiro Goto
IPC分类号： H01M4/86 , H01M8/10
CPC分类号： H01M4/8605 , H01M4/921 , H01M4/926 , H01M8/1011 , H01M2004/8684 , H01M2008/1095 , Y02E60/523
摘要： The present invention aims to provide a fuel cell anode, a membrane electrode assembly and a fuel cell, so as to obtain high electric power. The fuel cell anode has an electrode catalyst layer, and the electrode catalyst layer comprises a supported catalyst comprises electrically conductive carriers and fine catalytic particles supported thereon, a proton-conductive inorganic oxide supporting SiO2 on its surface, and a proton-conductive organic polymer binder. The SiO2 supported on the inorganic oxide prevents the oxide particles from growing, to ensure the high electric power. It is necessary to control the mixing ratios among the supported catalyst, the proton-conductive oxide and the proton-conductive binder in particular ranges.
摘要翻译：本发明旨在提供一种燃料电池阳极，膜电极组件和燃料电池，以获得高电力。燃料电池阳极具有电极催化剂层，电极催化剂层包括载体催化剂，其包含导电载体和负载在其上的细小催化剂颗粒，其表面上支持SiO 2的质子传导性无机氧化物和质子传导性有机聚合物粘合剂。负载在无机氧化物上的SiO2防止氧化物颗粒生长，确保高功率。需要在特定范围内控制负载型催化剂，质子传导性氧化物和质子传导性粘合剂的混合比例。

97. 发明申请

US20090325021A1 CATHODE FOR FUEL CELL 有权
标题翻译：燃料电池阴极
公开(公告)号：US20090325021A1
公开(公告)日：2009-12-31
申请号：US12372135
申请日：2009-02-17
申请人： Jun TAMURA , Yoshihiko Nakano
发明人： Jun TAMURA , Yoshihiko Nakano
IPC分类号： H01M4/86 , H01M8/10
CPC分类号： H01M4/8647 , H01M8/1004
摘要： A cathode for a fuel cell is provided, which includes an electrode catalyst layer. This electrode catalyst layer is constituted by a carried catalyst including a conductive carrier and catalytic fine particles carried on the conductive carrier, by a proton-conductive inorganic oxide containing an oxide carrier and oxide particles carried on a surface of the oxide carrier, and by a proton-conductive organic polymer binder. The carried catalyst is incorporated therein at a weight of WC. Silicon oxide is carried on the surface of the proton-conductive inorganic oxide at a weight ratio of 0.1-0.5 times as much as the weight of the proton-conductive inorganic oxide. The proton-conductive inorganic oxide is incorporated at a weight of WSA+SiO2. The weight ratio (WSA+SiO2/WC) is confined to 0.01-0.25. The proton-conductive organic polymer binder is incorporated at a weight of WP, the weigh ratio (WP/WSA+SiO2) is confined to 0.5-43.
摘要翻译：提供了一种用于燃料电池的阴极，其包括电极催化剂层。该电极催化剂层由携带有催化剂的催化剂构成，该催化剂包含导电性载体和载体在载体上的催化微粒，通过含有氧化物载体的质子传导性无机氧化物和承载在氧化物载体的表面上的氧化物粒子构成，质子传导性有机聚合物粘合剂。所携带的催化剂以WC的重量并入其中。氧化硅以质子传导性无机氧化物的重量的0.1-0.5倍的重量比承载在质子传导性无机氧化物的表面上。质子传导性无机氧化物以WSA + SiO 2的重量掺入。重量比（WSA + SiO2 / WC）限制在0.01-0.25。质子传导性有机聚合物粘合剂以WP的重量掺入，重量比（WP / WSA + SiO 2）被限制在0.5-43。

98. 发明申请

US20090247401A1 METHANOL OXIDATION CATALYST 有权
标题翻译：甲醇氧化催化剂
公开(公告)号：US20090247401A1
公开(公告)日：2009-10-01
申请号：US12401255
申请日：2009-03-10
申请人： Wu Mei , Taishi Fukazawa , Itsuko Mizutani , Tsuyoshi Kobayashi , Yoshihiko Nakano , Mina Farag , Shinji Aoki , Yi-Qun Li
发明人： Wu Mei , Taishi Fukazawa , Itsuko Mizutani , Tsuyoshi Kobayashi , Yoshihiko Nakano , Mina Farag , Shinji Aoki , Yi-Qun Li
IPC分类号： B01J23/42
CPC分类号： H01M4/921 , B01J21/18 , B01J23/6486 , B01J23/6525 , B01J23/6527 , B01J23/898 , B01J23/8993 , B01J35/006 , B82Y30/00 , C22C5/04 , H01M4/9041 , H01M4/925 , H01M4/926
摘要： A methanol oxidation catalyst comprises a material of composition: PtxMzTau in which Pt is platinum, Ta is tantalum, M is an element includes at least one selected from the group consisting of V (vanadium), W (tungsten), Ni (nickel) and Mo (molybdenum), x is 40 to 98 at. %, z is 1.5 to 55 at. %, and u is 0.5 to 40 at. %. To maximize catalytic activity the mater al is preferably in the form of nanoparticles. The values of x, z and u are selected such that the element exhibits X-ray photoelectron spectroscopy peaks derived from an oxygen bond and a metal bond in which a peak area derived from the oxygen bond is twice or less of a peak area derived from the metal bond.
摘要翻译：甲醇氧化催化剂包括组成的材料：<？in-line-formula description =“In-line Formulas”end =“lead”？> PtxMzTau <？in-line-formula description =“In-line Formulas”end = “尾”→其中Pt是铂，Ta是钽，M是元素包括选自V（钒），W（钨），Ni（镍）和Mo（钼），x 是40到98之间。％，z为1.5〜55at。％，u为0.5〜40at。％。为了最大限度地发挥催化活性，本发明优选为纳米颗粒的形式。选择x，z和u的值，使得该元件显示衍生自氧键和金属键的X射线光电子能谱峰，其中衍生自氧键的峰面积是衍生自氧键的峰面积的两倍或更少金属键。

99. 发明申请

US20090246589A1 FUEL CELL CATALYST, PROCESS FOR PREPARATION OF THE SAME, AND MEMBRANE ELECTRODE ASSEMBLY AND FUEL CELL EMPLOYING THE CATALYST 有权
标题翻译：燃料电池催化剂，其制备方法和膜电极组件和使用催化剂的燃料电池
公开(公告)号：US20090246589A1
公开(公告)日：2009-10-01
申请号：US12407076
申请日：2009-03-19
申请人： Taishi FUKAZAWA , Wu Mei , Yoshihiko Nakano , Tsuyoshi Kobayashi , Itsuko Mizutani , Hiroyasu Sumino
发明人： Taishi FUKAZAWA , Wu Mei , Yoshihiko Nakano , Tsuyoshi Kobayashi , Itsuko Mizutani , Hiroyasu Sumino
IPC分类号： H01M4/86 , H01M4/88 , B01J37/34
CPC分类号： H01M4/8867 , H01M4/8605 , H01M4/8871 , H01M4/8882 , H01M4/921 , H01M4/926 , H01M8/1007 , Y02P70/56
摘要： The present invention provides a catalyst having high activity and excellent stability, a process for preparation of the catalyst, a membrane electrode assembly, and a fuel cell. The catalyst of the present invention comprises an electronically conductive support and catalyst fine particles. The catalyst fine particles are supported on the support and are represented by the formula (1): PtuRuxGeyTz (1). In the formula, u, x, y and z mean 30 to 60 atm %, 20 to 50 atm %, 0.5 to 20 atm % and 0.5 to 40 atm %, respectively. When the element represented by T is Al, Si, Ni, W, Mo, V or C, the content of the T-element's atoms connected with oxygen bonds is not more than four times as large as that of the T-element's atoms connected with metal bonds on the basis of X-ray photoelectron spectrum (XPS) analysis. When the T-element is Ti, Hf, Sn, Ta, Zr or Nb, the content of the T-element's atoms connected with metal bonds is not more than twice as large as that of the T-element's atoms connected with oxygen bonds on the basis of XPS analysis.
摘要翻译：本发明提供了具有高活性和优异稳定性的催化剂，制备催化剂的方法，膜电极组件和燃料电池。本发明的催化剂包括电子导电载体和催化剂细颗粒。催化剂细颗粒负载在载体上，由式（1）表示：PtuRuxGeyTz（1）。在该式中，u，x，y和z分别表示30〜60atm％，20〜50atm％，0.5〜20atm％，0.5〜40atm％。当由T表示的元素是Al，Si，Ni，W，Mo，V或C时，与氧键连接的T元素原子的含量不超过T元素连接原子的含量的四倍在X射线光电子能谱（XPS）分析的基础上进行金属键合。当T元素是Ti，Hf，Sn，Ta，Zr或Nb时，与金属键连接的T元素原子的含量不超过与氧键连接的T元素原子的含量的两倍 XPS分析的基础。

100. 发明申请

US20090202887A1 CATALYST, ELECTRODE, MEMBRANE ELECTRODE ASSEMBLY AND FUEL CELL 有权
标题翻译：催化剂，电极，膜电极组件和燃料电池
公开(公告)号：US20090202887A1
公开(公告)日：2009-08-13
申请号：US12423313
申请日：2009-04-14
申请人： Tomoko Eguchi , Yoshihiko Nakano , Wu Mei , Taishi Fukazawa
发明人： Tomoko Eguchi , Yoshihiko Nakano , Wu Mei , Taishi Fukazawa
IPC分类号： H01M8/10
CPC分类号： H01M4/90 , H01M4/9075 , H01M4/921 , H01M4/925 , H01M8/1011 , H01M2004/8689 , Y02E60/523
摘要： Disclosed is a catalyst, including a catalyst particle containing at least one component selected from the group consisting of gold, platinum and an gold alloy, the gold alloy containing gold and at least one element selected from transition metal elements of the fourth period, fifth period and sixth period of the Periodic Table, and a catalyst carrier carrying the catalyst particle and containing a perovskite type oxide represented by general formula (1) given below: A(1-x)BxTiOy (1) where the element A is at least one element selected from the group consisting of Ca, Sr and Ba, the element B is at least one element selected from the group consisting of La, Nd, Sm, Eu, Gd, Dy, Ho, Er, Tm, Yb, and Lu, the molar ratio x satisfies 0
摘要翻译：公开了一种催化剂，其包括含有选自金，铂和金合金中的至少一种成分的催化剂颗粒，含有金的金合金和选自第四周期的第五期的过渡金属元素中的至少一种元素和第六周期，以及载有催化剂颗粒并含有由下式给出的通式（1）表示的钙钛矿型氧化物的催化剂载体：<？in-line-formula description =“In-line formula”end =“ 引线“→A（1-x）BxTiOy（1）<？在线公式描述=”在线公式“end =”tail“？>其中元素A是从以下组中选择的至少一种元素：的Ca，Sr和Ba中，元素B为选自La，Nd，Sm，Eu，Gd，Dy，Ho，Er，Tm，Yb和Lu中的至少一种元素，摩尔比x满足0

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