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91. 发明申请

US20100069660A1 PROCESS FOR PRODUCING GEOMETRIC SHAPED CATALYST BODIES 有权
标题翻译：生产几何形状催化剂体的方法
公开(公告)号：US20100069660A1
公开(公告)日：2010-03-18
申请号：US12557021
申请日：2009-09-10
申请人： Andreas Raichle , Catharina Horstmann , Frank Rosowski , Klaus Joachim Müller-Engel , Jochen Petzoldt , Ulrich Cremer
发明人： Andreas Raichle , Catharina Horstmann , Frank Rosowski , Klaus Joachim Müller-Engel , Jochen Petzoldt , Ulrich Cremer
IPC分类号： B01J21/06 , C07C45/27 , C07C255/00
CPC分类号： C07C51/252 , B01J23/002 , B01J23/8885 , B01J35/0006 , B01J35/023 , B01J37/0036 , B01J37/0221 , B01J37/34 , B01J2523/00 , C07C45/35 , C07C45/37 , C07C253/26 , Y02P20/52 , C07C47/22 , C07C57/04 , B01J2523/13 , B01J2523/41 , B01J2523/54 , B01J2523/68 , B01J2523/69 , B01J2523/842 , B01J2523/845 , C07C255/08
摘要： A process for producing geometric shaped catalyst bodies K whose active material is a multielement oxide of stoichiometry [BiaZ1bOx]p[BicMo12FedZ2eZ3fZ4gZ5hZ6iOy]1, in which a finely divided oxide BiaZ1bOx and, formed from element sources, a finely divided mixture of stoichiometry BicMo12FedZ2eZ3fZ4gZ5hZ6i are mixed in a ratio of p:1, this mixture is used to form shaped bodies and these are treated thermally, where 0
摘要翻译：用于生产几何形状的催化剂体K的方法，其活性材料是化学计量的多元素氧化物[BicMo12FedZ2eZ3fZ4gZ5hZ6iOy] 1，其中细分的氧化物BiaZ1bOx和由元素源形成的细分的化学计量比BicMo 12 FedZ 2eZ 3 fZ 4 gZ 5hZ 6i的混合物混合以p：1的比例，将该混合物用于形成成形体，并将它们热处理，其中0

92. 发明申请

US20090156835A1 PREPARATION OF PHTHALIC ANHYDRIDE BY GAS PHASE OXIDATION OF O-XYLENE IN A MAIN REACTOR AND POSTREACTOR 有权
标题翻译：通过气相氧化在主反应器和载体中制备邻苯二甲酸二异氰酸酯
公开(公告)号：US20090156835A1
公开(公告)日：2009-06-18
申请号：US12301370
申请日：2007-05-18
申请人： Thomas Mackewitz , Frank Rosowski , Andreas Tenten
发明人： Thomas Mackewitz , Frank Rosowski , Andreas Tenten
IPC分类号： C07D307/89
CPC分类号： C07D307/89 , C07C51/265 , C07C63/16
摘要： A process is described for preparing phthalic anhydride by catalytic gas phase oxidation of o-xylene, in which a gaseous mixture of o-xylene and an oxygenous gas is converted in a main reactor to a gaseous intermediate reaction product which comprises unconverted o-xylene, phthalic anhydride underoxidation products and phthalic anhydride, the heat of reaction which arises in the main reactor being removed at least partly by indirect cooling with a heat carrier medium, and the intermediate reaction product being introduced into a postreactor. The concentration of unconverted o-xylene in the intermediate reaction product is at least 1% by weight, and the sum of the concentrations of phthalic anhydride underoxidation products in the intermediate reaction product is at least 0.5% by weight. The process allows an increase in the overall yield of phthalic anhydride without or without significant deterioration in the product quality.
摘要翻译：描述了通过邻二甲苯的催化气相氧化制备邻苯二甲酸酐的方法，其中邻二甲苯和氧气的气体混合物在主反应器中转化为包含未转化的邻二甲苯的气态中间体反应产物，邻苯二甲酸酐脱氧产物和邻苯二甲酸酐，至少部分通过用载热介质间接冷却除去主反应器中产生的反应热，并将中间反应产物引入后反应器中。中间反应产物中未转化的邻二甲苯的浓度为至少1重量％，中间反应产物中邻苯二甲酸酐未氧化产物的浓度之和为至少0.5重量％。该方法允许邻苯二甲酸酐的总产率提高，而不会产生质量的显着劣化。

93. 发明申请

US20090118531A1 NOVEL SUPPORTED CATALYST FOR AMMOXIDATION 审中-公开
标题翻译：新型支持的氧化催化剂
公开(公告)号：US20090118531A1
公开(公告)日：2009-05-07
申请号：US12298806
申请日：2007-04-23
申请人： Hartmut Hibst , Sabine Huber , Frank Rosowski
发明人： Hartmut Hibst , Sabine Huber , Frank Rosowski
IPC分类号： C07C253/28 , B01J23/22
CPC分类号： B01J23/22 , B01J21/04 , B01J23/002 , B01J23/30 , B01J35/023 , B01J37/0201 , B01J37/0205 , B01J2523/00 , C07C253/28 , B01J2523/15 , B01J2523/53 , B01J2523/55 , B01J2523/69 , C07C255/51 , C07C255/50
摘要： Supported catalysts comprising a support having a mean diameter of ≦78 μm, a vanadium oxide, an antimony oxide, one or more alkali metal or alkaline earth metal oxides, and one or more oxides of tungsten, molybdenum, titanium, iron, cobalt, nickel, manganese, potassium, copper or mixtures thereof; processes for preparing said catalysts; and processes for preparing an aromatic or heteroaromatic nitrile in the presence of such a supported catalyst.
摘要翻译：包含平均直径<=78μm，氧化钒，氧化锑，一种或多种碱金属或碱土金属氧化物的载体和一种或多种钨，钼，钛，铁，钴，镍，锰，钾，铜或其混合物; 制备所述催化剂的方法; 以及在这种负载催化剂存在下制备芳族或杂芳族腈的方法。

94. 发明申请

US20080227992A1 Catalyst and Methods for Producing Maleic Anhydride 审中-公开
标题翻译：用于生产马来酸酐的催化剂和方法
公开(公告)号：US20080227992A1
公开(公告)日：2008-09-18
申请号：US11997023
申请日：2006-07-21
申请人： Cornelia Dobner , Mark Duda , Andreas Raichle , Hagen Wilmer , Frank Rosowski , Markus Holzle
发明人： Cornelia Dobner , Mark Duda , Andreas Raichle , Hagen Wilmer , Frank Rosowski , Markus Holzle
IPC分类号： C07D307/60 , B01J27/198 , B01J27/16
CPC分类号： B01J37/0009 , B01J23/002 , B01J23/8472 , B01J27/198 , B01J35/002 , B01J37/031 , B01J37/04 , B01J37/16 , B01J2523/00 , C07C51/215 , C07C57/145 , B01J2523/51 , B01J2523/55 , B01J2523/842
摘要： Catalysts comprising a catalytically active composition, the catalytically active composition comprising vanadium, phosphorus, iron and oxygen, wherein the catalytically active composition has an iron:vanadium atomic ratio of 0.005 to
摘要翻译：包含催化活性组合物的催化剂，包含钒，磷，铁和氧的催化活性组合物，其中催化活性组合物的铁：钒原子比为0.005至0.05，并且其中催化活性组合物中的铁衍生自铁原料，包含磷酸铁（III）; 并描述了制备这种催化剂的方法及其用途来制备马来酸酐。

95. 发明申请

US20080177105A1 PROCESS FOR PREPARING SHAPED CATALYST BODIES WHOSE ACTIVE COMPOSITION IS A MULTIELEMENT OXIDE 有权
标题翻译：活性成分为多种氧化物制备形成催化剂体的方法
公开(公告)号：US20080177105A1
公开(公告)日：2008-07-24
申请号：US12015741
申请日：2008-01-17
申请人： Andreas Raichle , Frank Rosowski , Sabine Huber , Ulrich Cremer , Stefan Altwasser , Klaus Joachim Mueller-Engel
发明人： Andreas Raichle , Frank Rosowski , Sabine Huber , Ulrich Cremer , Stefan Altwasser , Klaus Joachim Mueller-Engel
IPC分类号： C07C51/16 , C07C51/235 , C07C45/27 , B01J21/18 , B01J35/08
CPC分类号： B01J32/00 , B01J21/18 , B01J23/002 , B01J23/8885 , B01J27/186 , B01J37/0009 , B01J37/0018 , B01J2523/00 , C07C51/215 , C07C51/252 , C07C57/04 , C07C57/145 , B01J2523/13 , B01J2523/27 , B01J2523/41 , B01J2523/51 , B01J2523/54 , B01J2523/68 , B01J2523/842 , B01J2523/847 , B01J2523/845 , B01J2523/15 , B01J2523/17 , B01J2523/53 , B01J2523/55 , B01J2523/62 , B01J2523/69
摘要： A process for preparing shaped catalyst bodies whose active composition is a multielement oxide, in which a finely divided precursor mixture with addition of graphite having a specific particle size is shaped to the desired geometry and then treated thermally.
摘要翻译：一种制备活性组合物为多元素氧化物的成形催化剂体的方法，其中加入具有特定粒度的石墨的细碎前体混合物成形为所需几何形状，然后热处理。

96. 发明授权

US07271279B2 Method for the production of unsaturated nitriles from alkanes 失效
标题翻译：从烷烃生产不饱和腈的方法
公开(公告)号：US07271279B2
公开(公告)日：2007-09-18
申请号：US10482326
申请日：2002-06-25
申请人： Frieder Borgmeier , Frank Rosowski , Goetz-Peter Schindler
发明人： Frieder Borgmeier , Frank Rosowski , Goetz-Peter Schindler
IPC分类号： C07C253/18 , C07C255/08
CPC分类号： C07C253/26 , B01J27/199 , C07C45/33 , C07C45/35 , Y02P20/52 , C07C47/22 , C07C255/08
摘要： The invention relates to a process for preparing unsaturated nitrites from the corresponding alkanes which comprises the steps: a) feeding an alkane into a dehydrogenation zone and catalytically dehydrogenating the alkane to the corresponding alkene to obtain a product gas stream A which comprises the alkene, unconverted alkane and possibly one or more further gas components selected from the group consisting of steam, hydrogen, carbon oxides, hydrocarbons having a lower boiling point than the alkane or the alkene (low-boilers), nitrogen and noble gases, b) at least partially removing further gas components from the product gas stream A to give a feed gas stream B which comprises the alkane and the alkene, c) feeding the feed gas stream B, ammonia, an oxygen-containing gas and, if desired, steam into an oxidation zone and catalytically ammoxidizing the alkene to the corresponding unsaturated nitrile to give a product gas stream C which comprises the unsaturated nitrile, ammoxidation by-products, unconverted alkane and alkene and possibly one or more further gas components selected from the group consisting of steam, oxygen, carbon oxides, ammonia, nitrogen and noble gases, d) optionally removing ammonia from the product gas stream C to give an ammonia-depleted product gas stream D, e) removing the unsaturated nitrile and ammoxidation by-products from the product gas stream C or D by absorption in an aqueous absorbent to give a gas stream E which comprises unconverted alkane and alkene and possibly one or more further gas components selected from the group consisting of oxygen, carbon oxides, ammonia, nitrogen and noble gases, and an aqueous stream which comprises the nitrile and the by-products, and recovery of the unsaturated nitrile from the aqueous stream, f) recycling the gas stream E into the dehydrogenation zone.
摘要翻译：本发明涉及从相应的烷烃制备不饱和亚硝酸盐的方法，其包括以下步骤：a）将烷烃进料到脱氢区中，并将烷烃催化脱氢至相应的烯烃，得到产物气流A，其包含未转化的烯烃烷烃和可能的一种或多种另外的气体组分，其选自蒸汽，氢气，碳氧化物，沸点低于烷烃或烯烃（低沸点）的烃，氮气和惰性气体，b）至少部分从产物气流A中除去进一步的气体组分，得到包含烷烃和烯烃的进料气流B，c）将进料气流B，氨，含氧气体和如果需要的话进料到氧化物并将烯烃催化氨基化成相应的不饱和腈，得到包含不饱和腈的产物气流C，通过 - 产物，未转化的烷烃和烯烃以及可能的一种或多种另外的气体组分，其选自蒸汽，氧气，碳氧化物，氨，氮气和惰性气体，d）任选地从产物气流C除去氨，得到氨分离的产物气流D，e）通过在含水吸收剂中吸收从产物气流C或D中除去不饱和腈和氨氧化副产物，得到包含未转化的烷烃和烯烃的气流E，以及可能一个或多个另外的选自氧，碳氧化物，氨，氮和惰性气体的气体组分和包含腈和副产物的水流，以及从水流中回收不饱和腈，f）将气体再循环流E进入脱氢区。

97. 发明授权

US07253310B2 Preparation of (meth)acrylic acid 有权
标题翻译：（甲基）丙烯酸的制备
公开(公告)号：US07253310B2
公开(公告)日：2007-08-07
申请号：US10920428
申请日：2004-08-18
申请人： Frieder Borgmeier , Frank Rosowski , Hans-Guenther Lintz , Ina Grisstede , Elisabet Bacells Cabre
发明人： Frieder Borgmeier , Frank Rosowski , Hans-Guenther Lintz , Ina Grisstede , Elisabet Bacells Cabre
IPC分类号： C07C51/16
CPC分类号： C07C51/215 , C07C57/04
摘要： A process for preparing (meth)acrylic acid by heterogeneously catalyzed gas phase partial oxidation of a saturated hydrocarbon precursor compound, in which the charging gas mixture contains from 5 to 25% by volume of steam and the molar ratio of molecular oxygen present in the charging gas mixture to saturated hydrocarbon precursor compound present in the charging gas mixture is from 1.5:1 to 2.5:1.
摘要翻译：一种通过饱和烃前体化合物的非均相催化气相部分氧化制备（甲基）丙烯酸的方法，其中装料气体混合物含有5至25体积％的蒸汽和在充料中存在的分子氧的摩尔比与充填气体混合物中存在的饱和烃前体化合物的气体混合物为1.5:1至2.5:1。

98. 发明授权

US07019169B2 Preparation of (meth)acrylic acid 失效
标题翻译：（甲基）丙烯酸的制备
公开(公告)号：US07019169B2
公开(公告)日：2006-03-28
申请号：US10934442
申请日：2004-09-07
申请人： Frieder Borgmeier , Frank Rosowski , Hans-Günther Lintz , Ina Grisstede
发明人： Frieder Borgmeier , Frank Rosowski , Hans-Günther Lintz , Ina Grisstede
IPC分类号： C07C51/16
CPC分类号： C07C51/215 , C07C57/04
摘要： A process for preparing (meth)acrylic acid by conducting a saturated hydrocarbon precursor compound through a catalyst bed I whose catalysts I have, as the active composition, a multimetal oxide I which has a specific X-ray diffractogram and contains the elements Mo and V, at least one of the elements Te and Sb, and also at least one of the elements from the group consisting of Nb, Ta, W, Ce and Ti, wherein the catalyst bed I is interrupted by at least one catalyst bed II whose catalysts II have, as the active composition, a multimetal oxide II which contains the elements Mo, Bi and Fe.
摘要翻译：通过使催化剂床I（其具有催化剂床I）作为活性组合物，通过具有特定的X射线衍射图并含有元素Mo和V的多金属氧化物I来导入饱和烃前体化合物来制备（甲基）丙烯酸的方法，元素Te和Sb中的至少一种，以及来自Nb，Ta，W，Ce和Ti的元素中的至少一种元素，其中催化剂床I被至少一个催化剂床II中断，催化剂床II的催化剂床作为活性组合物，II具有包含元素Mo，Bi和Fe的多金属氧化物II。

99. 发明申请

US20050065372A1 Preparation of (meth)acrylic acid 失效
标题翻译：（甲基）丙烯酸的制备
公开(公告)号：US20050065372A1
公开(公告)日：2005-03-24
申请号：US10934624
申请日：2004-09-07
申请人： Frieder Borgmeier , Frank Rosowski , Hans Martan , Klaus Muller-Engel
发明人： Frieder Borgmeier , Frank Rosowski , Hans Martan , Klaus Muller-Engel
IPC分类号： B01J23/00 , B01J23/28 , B01J23/887 , B01J27/057 , B01J35/00 , B01J37/00 , C07C51/215 , C07C51/16 , C07C51/235
CPC分类号： C07C51/215 , B01J23/002 , B01J23/28 , B01J23/8877 , B01J27/0576 , B01J35/0006 , B01J37/0045 , B01J2523/00 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , B01J2523/847 , B01J2523/32
摘要： A process for preparing (meth)acrylic acid, in which a saturated hydrocarbon precursor compound is conducted through a catalyst charge which consists of two spatially successive catalyst beds I, II in the flow direction of the reaction mixture, each of which contains different catalysts and has different reaction-selectivity behavior.
摘要翻译：一种制备（甲基）丙烯酸的方法，其中饱和烃前体化合物通过催化剂装料进行，催化剂装料由反应混合物流动方向上的两个空间连续的催化剂床I，II组成，每个催化剂床含有不同的催化剂和具有不同的反应选择性行为。

100. 发明申请

US20050043567A1 Preparation of (meth)acrylic acid 有权
标题翻译：（甲基）丙烯酸的制备
公开(公告)号：US20050043567A1
公开(公告)日：2005-02-24
申请号：US10920428
申请日：2004-08-18
申请人： Frieder Borgmeier , Frank Rosowski , Hans-Gunther Lintz , Ina Grisstede , Elisabet Cabre
发明人： Frieder Borgmeier , Frank Rosowski , Hans-Gunther Lintz , Ina Grisstede , Elisabet Cabre
IPC分类号： C07C51/215 , C07C51/16 , C07C51/235
CPC分类号： C07C51/215 , C07C57/04
摘要： A process for preparing (meth)acrylic acid by heterogeneously catalyzed gas phase partial oxidation of a saturated hydrocarbon precursor compound, in which the charging gas mixture contains from 5 to 25% by volume of steam and the molar ratio of molecular oxygen present in the charging gas mixture to saturated hydrocarbon precursor compound present in the charging gas mixture is from 1.5:1 to 2.5:1.
摘要翻译：一种通过饱和烃前体化合物的非均相催化气相部分氧化制备（甲基）丙烯酸的方法，其中装料气体混合物含有5至25体积％的蒸汽和在充料中存在的分子氧的摩尔比与充填气体混合物中存在的饱和烃前体化合物的气体混合物为1.5:1至2.5:1。

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