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91. 发明申请

US20100029975A1 Integrated process for preparing a carboxylic acid from an alkane 审中-公开
标题翻译：从烷烃制备羧酸的综合方法
公开(公告)号：US20100029975A1
公开(公告)日：2010-02-04
申请号：US12459970
申请日：2009-07-10
申请人： Scott Han , Wolfgang Ruettinger , Douglass W. Sevon
发明人： Scott Han , Wolfgang Ruettinger , Douglass W. Sevon
IPC分类号： C07C253/00 , C07C51/16
CPC分类号： C07C51/252 , Y02P20/125 , Y02P20/51 , Y02P20/582 , C07C57/04
摘要： The present invention relates to an integrated process for producing unsaturated carboxylic acids from the corresponding C2-C4 alkane. The process begins with integrated catalytic reactions comprising endothermic soft oxidant conversion (SOC) and exothermic selective hydrogen combustion (SHC) which cumulatively convert a C2-C4 alkane to its corresponding C2-C4 alkene in a product stream substantially free of hydrogen. Heat from the exothermic selective hydrogen combustion reaction zone is recovered and recycled back upstream to the endothermic soft oxidant conversion reaction zone. The hydrogen-free alkene products of the thermally integrated SOC/SHC reactions are then provided to a catalytic vapor phase partial oxidation process for conversion of the alkene to the corresponding unsaturated carboxylic acid or nitrile. Unreacted alkene and carbon dioxide are recovered from the oxidation product stream and recycled back to the thermally integrated soft oxidant conversion reactions.
摘要翻译：本发明涉及从相应的C 2 -C 4烷烃制备不饱和羧酸的综合方法。该过程开始于包括吸热软氧化剂转化（SOC）和放热选择性氢燃烧（SHC）的综合催化反应，其在基本上不含氢的产物流中将C 2 -C 4烷烃累加转化成其相应的C 2 -C 4烯烃。来自放热选择性氢燃烧反应区的热量被回收并循环回到吸热软氧化剂转化反应区的上游。然后将热集成的SOC / SHC反应的无氢烯烃产物提供到用于将烯烃转化成相应的不饱和羧酸或腈的催化气相部分氧化方法。从氧化产物流中回收未反应的烯烃和二氧化碳，并循环回热积分的软氧化剂转化反应。

92. 发明申请

US20090182186A1 Supported catalyst for conversion of propane to propene and its use in a process for that conversion 审中-公开
标题翻译：用于将丙烷转化成丙烯的载体催化剂及其在该转化过程中的用途
公开(公告)号：US20090182186A1
公开(公告)日：2009-07-16
申请号：US12319765
申请日：2009-01-12
申请人： Abraham Benderly , Wolfgang Ruettinger , Scott Han
发明人： Abraham Benderly , Wolfgang Ruettinger , Scott Han
IPC分类号： C07C5/32
CPC分类号： B01J23/685 , B01J21/08 , B01J23/26 , B01J35/1019 , B01J35/1023 , B01J35/1028 , B01J35/1061 , B01J35/1066 , B01J37/0201 , C07C5/3332 , C07C5/42 , C07C2521/06 , C07C2521/08 , C07C2523/06 , C07C2523/10 , C07C2523/22 , C07C2523/26 , C07C2523/28 , C07C2523/50 , Y02P20/52 , C07C11/06
摘要： A process for the conversion of propane to propene is disclosed wherein a silica chromium catalyst composition is contacted with a propane feed stream and a carbon dioxide. The silica chromium catalyst composition is further disclosed wherein the composition, optionally, includes a promoter component.
摘要翻译：公开了一种将丙烷转化为丙烯的方法，其中将二氧化硅铬催化剂组合物与丙烷进料流和二氧化碳接触。进一步公开了二氧化硅铬催化剂组合物，其中组合物任选地包含促进剂组分。

93. 发明申请

US20080154056A1 Process for the selective (AMM) oxidation of lower molecular weight alkanes and alkenes 有权
标题翻译：低分子量烷烃和烯烃的选择性（AMM）氧化方法
公开(公告)号：US20080154056A1
公开(公告)日：2008-06-26
申请号：US11985671
申请日：2007-11-16
申请人： Anne Mae Gaffney , Scott Han
发明人： Anne Mae Gaffney , Scott Han
IPC分类号： C07C51/16 , C07C255/07 , C07C255/03
CPC分类号： C07C253/24 , C07C51/215 , C07C51/252 , C07C51/43 , Y02P20/52 , Y02P20/582 , C07C57/04 , C07C255/08
摘要： An improved process for the production of unsaturated carboxylic acids and unsaturated nitriles from their corresponding C3 to C5 alkanes, or mixtures of C3 to C5 alkanes and alkenes, that involves oxidation in the presence of a supported Mo-V-based mixed metal oxide catalyst in a multi-stage reaction system which employs both separation of the oxidation product from one or more intermediate effluent streams, as well as feeding additional oxygen to reaction zones subsequent to the first reaction zone.
摘要翻译：用于从相应的C 3至C 5烷烃生产不饱和羧酸和不饱和腈的改进方法，或C 3 - 3 - 的混合物与 C 5烷烃和烯烃，其包括在多阶段反应体系中在负载的Mo-V基混合金属氧化物催化剂存在下进行氧化，该多级反应体系采用将氧化产物从一种或多种中间流出物流，以及在第一反应区之后的反应区域中加入额外的氧气。

94. 发明授权

US07326668B2 Single crystalline phase catalyst 失效
标题翻译：单晶相催化剂
公开(公告)号：US07326668B2
公开(公告)日：2008-02-05
申请号：US11640686
申请日：2006-12-18
申请人： Leonard Edward Bogan, Jr. , Daniel A. Bors , Fernando Antonio Pessoa Cavalcanti , Michael Bruce Clark, Jr. , Anne Mae Gaffney , Scott Han
发明人： Leonard Edward Bogan, Jr. , Daniel A. Bors , Fernando Antonio Pessoa Cavalcanti , Michael Bruce Clark, Jr. , Anne Mae Gaffney , Scott Han
IPC分类号： B01J23/00 , B01J23/20 , C07C253/00
CPC分类号： C07C51/215 , B01J23/002 , B01J23/20 , B01J23/28 , B01J27/0576 , B01J37/0236 , B01J37/08 , B01J2523/00 , C07C51/252 , C07C253/24 , C07C253/26 , Y02P20/52 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , C07C255/08
摘要： An orthorhombic phase mixed metal oxide is produced selectively in quantitative yield and used to produce.
摘要翻译：选择性地以定量收率生产正交相混合金属氧化物，并用于生产。

95. 发明申请

US20070179042A1 Regenerated mixed metal oxide catalysts 有权
标题翻译：再生混合金属氧化物催化剂
公开(公告)号：US20070179042A1
公开(公告)日：2007-08-02
申请号：US11650909
申请日：2007-01-08
申请人： Fernando Antonio Pessoa Cavalcanti , Scott Han , Peter David Klugherz , Andrew Michael Lemonds , Daniel J. Martenak , Elsie Mae Vickery , Donald Lee Zolotorofe
发明人： Fernando Antonio Pessoa Cavalcanti , Scott Han , Peter David Klugherz , Andrew Michael Lemonds , Daniel J. Martenak , Elsie Mae Vickery , Donald Lee Zolotorofe
IPC分类号： B01J20/34
CPC分类号： B01J23/002 , B01J23/28 , B01J23/30 , B01J23/6525 , B01J23/92 , B01J23/96 , B01J27/0576 , B01J27/30 , B01J35/002 , B01J37/0236 , B01J37/0238 , B01J37/342 , B01J38/04 , B01J38/06 , B01J38/08 , B01J38/16 , B01J2523/00 , C07C51/215 , C07C253/24 , Y02P20/52 , Y02P20/584 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , B01J2523/824 , C07C255/08
摘要： A mixed metal oxide, which may be an orthorhombic phase material, is regenerated, selectively enriched or selectively poisoned as a catalyst to reduce catalyst aging for the production of unsaturated carboxylic acids, or unsaturated nitrites, from alkanes, or mixtures of alkanes and alkenes, by contacting said mixed metal oxide with a an oxidizing gas such as oxygen, air, steam and combinations thereof is permitted to flow through the catalyst in a regenerator at a temperature of from 300° C. to 600° C. to form said regenerated catalyst.
摘要翻译：可以是正交相材料的混合金属氧化物被再生，选择性地富集或选择性地中毒作为催化剂，以减少催化剂老化，用于从烷烃或烷烃和烯烃的混合物生产不饱和羧酸或不饱和腈，通过使所述混合金属氧化物与氧气，空气，蒸汽及其组合的氧化气体接触，可以在300℃至600℃的温度下在再生器中流过催化剂以形成所述再生催化剂。

96. 发明申请

US20060122055A1 (Amm)oxidation catalyst and catalytic (amm)oxidation process for conversion of lower alkanes 审中-公开
标题翻译：（Amm）氧化催化剂和催化（amm）氧化方法转化低级烷烃
公开(公告)号：US20060122055A1
公开(公告)日：2006-06-08
申请号：US11272629
申请日：2005-11-14
申请人： Anne Gaffney , John Gleaves , Scott Han , Ruozhi Song
发明人： Anne Gaffney , John Gleaves , Scott Han , Ruozhi Song
IPC分类号： B01J27/187 , B01J27/198 , B01J27/188 , B01J23/00 , B01J27/185 , B01J27/192 , B01J27/19
CPC分类号： C07C51/215 , B01J23/002 , B01J23/28 , B01J27/0576 , B01J35/002 , B01J37/0238 , B01J2523/00 , Y02P20/582 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68
摘要： The present invention relates to mixed metal oxide (MMO1) catalysts. MMO1 catalyst performance is improved with a sub-monolayer deposition of Te onto its surface by vapor deposition. The selectivity to acrylic acid improved by approximately 6% and the acrylic acid yield by 3%, absolute. Applying a similar Te loading onto MMO1 by wet impregnation methods did not improve catalytic performance. Post treatment of the Te vapor deposited MMO1 catalyst with oxygen at elevated temperatures gave improved catalytic performance when compared to a corresponding sample treated with an inert gas at the same elevated temperatures.
摘要翻译：本发明涉及混合金属氧化物（MMO1）催化剂。通过气相沉积在其表面上通过亚单层沉积Te来改善MMO1催化剂性能。丙烯酸的选择性提高约6％，丙烯酸收率提高3％，绝对值。通过湿式浸渍法将类似的Te载体施加到MMO1上并没有改善催化性能。与在相同高温下用惰性气体处理的相应样品相比，在升高的温度下用Te气相沉积的MMO1催化剂后处理提供了改进的催化性能。

97. 发明授权

US06965050B2 Single crystalline phase catalyst 失效
公开(公告)号：US06965050B2
公开(公告)日：2005-11-15
申请号：US10807069
申请日：2004-03-23
申请人： Leonard Edward Bogan, Jr. , Daniel A. Bors , Fernando Antonio Pessoa Cavalcanti , Michael Bruce Clark, Jr. , Anne Mae Gaffney , Scott Han
发明人： Leonard Edward Bogan, Jr. , Daniel A. Bors , Fernando Antonio Pessoa Cavalcanti , Michael Bruce Clark, Jr. , Anne Mae Gaffney , Scott Han
IPC分类号： C01G39/00 , B01J23/00 , B01J23/20 , B01J23/28 , B01J23/887 , B01J27/057 , B01J37/02 , B01J37/04 , B01J37/08 , C07B61/00 , C07C51/16 , C07C51/215 , C07C57/05 , C07C253/24 , C07C253/26 , C07C255/08
CPC分类号： C07C51/215 , B01J23/002 , B01J23/20 , B01J23/28 , B01J27/0576 , B01J37/0236 , B01J37/08 , B01J2523/00 , C07C51/252 , C07C253/24 , C07C253/26 , Y02P20/52 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , C07C255/08
摘要： An orthorhombic phase mixed metal oxide is produced selectively in quantitative yield.

98. 发明授权

US06911556B2 Processes for the preparation of olefins, unsaturated carboxylic acids and unsaturated nitriles from alkanes 失效
标题翻译：从烷烃制备烯烃，不饱和羧酸和不饱和腈的方法
公开(公告)号：US06911556B2
公开(公告)日：2005-06-28
申请号：US10712744
申请日：2003-11-13
申请人： Leonard Edward Bogan, Jr. , Anne Mae Gaffney , Scott Han , Michele Doreen Heffner , Ruozhi Song , Donald Lee Zolotorofe
发明人： Leonard Edward Bogan, Jr. , Anne Mae Gaffney , Scott Han , Michele Doreen Heffner , Ruozhi Song , Donald Lee Zolotorofe
IPC分类号： C07C5/48 , C07B61/00 , C07C11/06 , C07C51/21 , C07C57/05 , C07C235/24 , C07C253/24 , C07C255/08 , C07C51/16
CPC分类号： C07C253/24 , B01J21/066 , B01J23/28 , B01J23/868 , B01J23/8993 , B01J35/04 , B01J37/0201 , B01J2523/00 , Y02P20/52 , C07C255/08 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , B01J2523/27 , B01J2523/31
摘要： Improved processes for the preparation of olefins, unsaturated carboxylic acids and unsaturated nitriles involve the use of dehydrogenation catalysts suitable for the conversion of alkanes to alkenes and catalysts suitable for the conversion of alkanes and/or alkenes to unsaturated carboxylic acids or unsaturated nitriles.
摘要翻译：用于制备烯烃，不饱和羧酸和不饱和腈的改进方法包括使用适于将烷烃转化为烯烃的脱氢催化剂和适用于将烷烃和/或烯烃转化为不饱和羧酸或不饱和腈的催化剂。

99. 发明申请

US20050131255A1 Catalyst systems for converting alkanes to alkenes and to their corresponding oxygenated products 审中-公开
标题翻译：将烷烃转化为烯烃及其相应的氧化产物的催化剂体系
公开(公告)号：US20050131255A1
公开(公告)日：2005-06-16
申请号：US10987367
申请日：2004-11-12
申请人： Abraham Benderly , Nitin Chadda , Anne Gaffney , Scott Han , Dominique Le , Mark Silvano
发明人： Abraham Benderly , Nitin Chadda , Anne Gaffney , Scott Han , Dominique Le , Mark Silvano
IPC分类号： B01J23/887 , B01J23/00 , B01J23/38 , B01J23/54 , B01J23/62 , B01J23/648 , B01J23/652 , B01J23/76 , B01J27/057 , B01J27/14 , B01J35/00 , B01J35/04 , B01J37/00 , B01J37/02 , B01J37/08 , C07B61/00 , C07C5/327 , C07C5/333 , C07C5/48 , C07C11/06 , C07C51/16 , C07C51/215 , C07C53/122 , C07C57/05 , C07C67/39
CPC分类号： B01J35/0006 , B01J23/002 , B01J23/54 , B01J23/62 , B01J23/6484 , B01J23/6525 , B01J27/0576 , B01J35/04 , B01J37/0036 , B01J37/0215 , B01J2523/00 , C07C5/3335 , C07C5/3337 , C07C51/215 , C07C67/39 , C07C2521/04 , C07C2523/62 , C07C2523/648 , C07C11/02 , C07C57/04 , B01J2523/31 , B01J2523/56 , B01J2523/828 , B01J2523/55 , B01J2523/64 , B01J2523/68 , B01J2523/824 , B01J2523/33 , C07C69/54
摘要： Alkenes, unsaturated saturated carboxylic acids, saturated carboxylic acids and their higher analogues are prepared directly from corresponding alkanes utilizing using a mixed bed catalyst at flame temperatures in a short contact time reactor.
摘要翻译：烯烃，不饱和饱和羧酸，饱和羧酸及其较高的类似物，可以在短时间接触时间反应器中，在火焰温度下使用混合床催化剂直接从相应的烷烃制备。

100. 发明授权

US06841699B2 Recalcined catalyst 有权
标题翻译：再煅烧催化剂
公开(公告)号：US06841699B2
公开(公告)日：2005-01-11
申请号：US10117908
申请日：2002-04-08
申请人： Leonard Edward Bogan, Jr. , Anne Mae Gaffney , Scott Han , Michele Doreen Heffner , Ruozhi Song
发明人： Leonard Edward Bogan, Jr. , Anne Mae Gaffney , Scott Han , Michele Doreen Heffner , Ruozhi Song
IPC分类号： C01B19/00 , B01J23/00 , B01J23/20 , B01J23/28 , B01J23/887 , B01J27/057 , B01J37/02 , B01J37/06 , B01J37/08 , C07B61/00 , C07C51/215 , C07C51/25 , C07C57/05 , C07C253/24 , C07C253/26 , C07C255/08
CPC分类号： C07C51/215 , B01J23/002 , B01J23/20 , B01J23/28 , B01J27/0576 , B01J37/0236 , B01J37/06 , B01J37/08 , B01J2523/00 , C07C253/24 , C07C253/26 , Y02P20/52 , C07C57/04 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , C07C255/08
摘要： A mixed metal oxide, which may be an orthorhombic phase material, is improved as a catalyst for the production of unsaturated carboxylic acids, or unsaturated nitriles, from alkanes, or mixtures of alkanes and alkenes, by: contacting with a liquid contacting member selected from the group consisting of organic acids, alcohols, inorganic acids and hydrogen peroxide to form a contact mixture; recovering insoluble material from the contact mixture; and calcining the recovered insoluble material in a non-oxidizing atmosphere.
摘要翻译：可以作为斜方相材料的混合金属氧化物作为用于通过以下方式与烷烃或烯烃的混合物生产不饱和羧酸或不饱和腈的催化剂进行改进：由有机酸，醇，无机酸和过氧化氢组成的组合形成接触混合物; 从接触混合物中回收不溶物质; 并将回收的不溶物质煅烧在非氧化性气氛中。

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